Atomically thin materials are exceedingly susceptible to their dielectric environment. For transition metal dichalcogenides, sample placement on a substrate or encapsulation in hexagonal boron nitride (hBN) are frequently used. In this paper we show that the dielectric response due to optical phonons of adjacent materials influences excitons in two-dimensional (2D) crystals. We provide an analytic model for the coupling of 2D charge carriers to optical substrate phonons, which causes polaron effects similar to that of intrinsic 2D phonons. We apply the model to hBN-encapsulated WSe2, finding a significant reduction of the exciton binding energies due to dynamical screening effects.
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Baugher BWH, 2014, NAT NANOTECHNOL, V9, P262, DOI [10.1038/nnano.2014.25, 10.1038/NNANO.2014.25]
机构:
Friedrich Schiller Univ Jena, Inst Festkorpertheorie & Opt, Max Wien Pl 1, D-07743 Jena, Germany
Friedrich Schiller Univ Jena, European Theoret Spect Facil, Max Wien Pl 1, D-07743 Jena, GermanyFriedrich Schiller Univ Jena, Inst Festkorpertheorie & Opt, Max Wien Pl 1, D-07743 Jena, Germany
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Chernikov, Alexey
;
Berkelbach, Timothy C.
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Chem, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Berkelbach, Timothy C.
;
Hill, Heather M.
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Hill, Heather M.
;
Rigosi, Albert
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Rigosi, Albert
;
Li, Yilei
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Li, Yilei
;
Aslan, Ozgur Burak
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Aslan, Ozgur Burak
;
Reichman, David R.
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Chem, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Reichman, David R.
;
Hybertsen, Mark S.
论文数: 0引用数: 0
h-index: 0
机构:
Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Hybertsen, Mark S.
;
Heinz, Tony F.
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
机构:
Univ Washington, Dept Phys, Seattle, WA 98195 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA
Chow, Colin M.
;
Yu, Hongyi
论文数: 0引用数: 0
h-index: 0
机构:
Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China
Univ Hong Kong, Ctr Theoret & Computat Phys, Hong Kong, Hong Kong, Peoples R ChinaUniv Washington, Dept Phys, Seattle, WA 98195 USA
Yu, Hongyi
;
Jones, Aaron M.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Washington, Dept Phys, Seattle, WA 98195 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA
Jones, Aaron M.
;
Yan, Jiaqiang
论文数: 0引用数: 0
h-index: 0
机构:
Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA
Yan, Jiaqiang
;
Mandrus, David G.
论文数: 0引用数: 0
h-index: 0
机构:
Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA
Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA
Mandrus, David G.
;
Taniguchi, Takashi
论文数: 0引用数: 0
h-index: 0
机构:
Natl Inst Mat Sci, Adv Mat Lab, Tsukuba, Ibaraki, JapanUniv Washington, Dept Phys, Seattle, WA 98195 USA
Taniguchi, Takashi
;
Watanabe, Kenji
论文数: 0引用数: 0
h-index: 0
机构:
Natl Inst Mat Sci, Adv Mat Lab, Tsukuba, Ibaraki, JapanUniv Washington, Dept Phys, Seattle, WA 98195 USA
Watanabe, Kenji
;
Yao, Wang
论文数: 0引用数: 0
h-index: 0
机构:
Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China
Univ Hong Kong, Ctr Theoret & Computat Phys, Hong Kong, Hong Kong, Peoples R ChinaUniv Washington, Dept Phys, Seattle, WA 98195 USA
Yao, Wang
;
Xu, Xiaodong
论文数: 0引用数: 0
h-index: 0
机构:
Univ Washington, Dept Phys, Seattle, WA 98195 USA
Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA
机构:
Friedrich Schiller Univ Jena, Inst Festkorpertheorie & Opt, Max Wien Pl 1, D-07743 Jena, Germany
Friedrich Schiller Univ Jena, European Theoret Spect Facil, Max Wien Pl 1, D-07743 Jena, GermanyFriedrich Schiller Univ Jena, Inst Festkorpertheorie & Opt, Max Wien Pl 1, D-07743 Jena, Germany
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Chernikov, Alexey
;
Berkelbach, Timothy C.
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Chem, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Berkelbach, Timothy C.
;
Hill, Heather M.
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Hill, Heather M.
;
Rigosi, Albert
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Rigosi, Albert
;
Li, Yilei
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Li, Yilei
;
Aslan, Ozgur Burak
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Aslan, Ozgur Burak
;
Reichman, David R.
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Chem, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Reichman, David R.
;
Hybertsen, Mark S.
论文数: 0引用数: 0
h-index: 0
机构:
Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
Hybertsen, Mark S.
;
Heinz, Tony F.
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Univ, Dept Phys, New York, NY 10027 USA
Columbia Univ, Dept Elect Engn, New York, NY 10027 USAColumbia Univ, Dept Phys, New York, NY 10027 USA
机构:
Univ Washington, Dept Phys, Seattle, WA 98195 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA
Chow, Colin M.
;
Yu, Hongyi
论文数: 0引用数: 0
h-index: 0
机构:
Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China
Univ Hong Kong, Ctr Theoret & Computat Phys, Hong Kong, Hong Kong, Peoples R ChinaUniv Washington, Dept Phys, Seattle, WA 98195 USA
Yu, Hongyi
;
Jones, Aaron M.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Washington, Dept Phys, Seattle, WA 98195 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA
Jones, Aaron M.
;
Yan, Jiaqiang
论文数: 0引用数: 0
h-index: 0
机构:
Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA
Yan, Jiaqiang
;
Mandrus, David G.
论文数: 0引用数: 0
h-index: 0
机构:
Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA
Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA
Mandrus, David G.
;
Taniguchi, Takashi
论文数: 0引用数: 0
h-index: 0
机构:
Natl Inst Mat Sci, Adv Mat Lab, Tsukuba, Ibaraki, JapanUniv Washington, Dept Phys, Seattle, WA 98195 USA
Taniguchi, Takashi
;
Watanabe, Kenji
论文数: 0引用数: 0
h-index: 0
机构:
Natl Inst Mat Sci, Adv Mat Lab, Tsukuba, Ibaraki, JapanUniv Washington, Dept Phys, Seattle, WA 98195 USA
Watanabe, Kenji
;
Yao, Wang
论文数: 0引用数: 0
h-index: 0
机构:
Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China
Univ Hong Kong, Ctr Theoret & Computat Phys, Hong Kong, Hong Kong, Peoples R ChinaUniv Washington, Dept Phys, Seattle, WA 98195 USA
Yao, Wang
;
Xu, Xiaodong
论文数: 0引用数: 0
h-index: 0
机构:
Univ Washington, Dept Phys, Seattle, WA 98195 USA
Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USAUniv Washington, Dept Phys, Seattle, WA 98195 USA