Near-field probing of image phonon-polaritons in hexagonal boron nitride on gold crystals

被引:24
作者
Menabde, Sergey G. [1 ]
Boroviks, Sergejs [2 ,3 ]
Ahn, Jongtae [4 ]
Heiden, Jacob T. [1 ]
Watanabe, Kenji [5 ]
Taniguchi, Takashi [6 ]
Low, Tony [7 ]
Hwang, Do Kyung [3 ,8 ]
Mortensen, N. Asger [2 ,9 ]
Jang, Min Seok [1 ]
机构
[1] Korea Adv Inst Sci & Technol, Sch Elect Engn, Daejeon, South Korea
[2] Univ Southern Denmark, Ctr Nano Opt, Odense, Denmark
[3] Swiss Fed Inst Technol Lausanne EPFL, Nanophoton & Metrol Lab, Lausanne, Switzerland
[4] Korea Inst Sci & Technol, Ctr Optoelect Mat & Devices, Seoul, South Korea
[5] Natl Inst Mat Sci, Res Ctr Funct Mat, Tsukuba, Ibaraki, Japan
[6] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton, Tsukuba, Ibaraki, Japan
[7] Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN USA
[8] Univ Sci & Technol, Div Nano & Informat Technol, Daejeon, South Korea
[9] Univ Southern Denmark, Danish Inst Adv Study, Odense, Denmark
基金
新加坡国家研究基金会;
关键词
CONFINED POLARITONS; PLASMONS;
D O I
10.1126/sciadv.abn0627
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Near-field mapping has been widely used to study hyperbolic phonon-polaritons in van der Waals crystals. However, an accurate measurement of the polaritonic loss remains challenging because of the inherent complexity of the near-field signal and the substrate-mediated loss. Here we demonstrate that large-area monocrystalline gold flakes, an atomically flat low-loss substrate for image polaritons, provide a platform for precise near-field measurement of the complex propagation constant of polaritons in van der Waals crystals. As a topical example, we measure propagation loss of the image phonon-polaritons in hexagonal boron nitride, revealing that their normalized propagation length exhibits a parabolic spectral dependency. Furthermore, we show that image phononpolaritons exhibit up to a twice longer normalized propagation length, while being 2.4 times more compressed compared to the case of the dielectric substrate. We conclude that the monocrystalline gold flakes provide a unique nanophotonic platform for probing and exploitation of the image modes in low-dimensional materials.
引用
收藏
页数:6
相关论文
共 36 条
[1]   Probing the ultimate plasmon confinement limits with a van der Waals heterostructure [J].
Alcaraz Iranzo, David ;
Nanot, Sebastien ;
Dias, Eduardo J. C. ;
Epstein, Itai ;
Peng, Cheng ;
Efetov, Dmitri K. ;
Lundeberg, Mark B. ;
Parret, Romain ;
Osmond, Johann ;
Hong, Jin-Yong ;
Kong, Jing ;
Englund, Dirk R. ;
Peres, Nuno M. R. ;
Koppens, Frank H. L. .
SCIENCE, 2018, 360 (6386) :291-295
[2]   Infrared Permittivity of the Biaxial van der Waals Semiconductor α-MoO3 from Near- and Far-Field Correlative Studies [J].
Alvarez-Perez, Gonzalo ;
Foland, Thomas G. ;
Errea, Ion ;
Taboada-Gutierrez, Javier ;
Duan, Jiahua ;
Martin-Sanchez, Javier ;
Tresguerres-Mata, Ana I. F. ;
Matson, Joseph R. ;
Bylinkin, Andrei ;
He, Mingze ;
Ma, Weiliang ;
Bao, Qiaoliang ;
Ignacio Martin, Jose ;
Caldwell, Joshua D. ;
Nikitin, Alexey Y. ;
Alonso-Gonzalez, Pablo .
ADVANCED MATERIALS, 2020, 32 (29)
[3]   Analytical approximations for the dispersion of electromagnetic modes in slabs of biaxial crystals [J].
Alvarez-Perez, Gonzalo ;
Voronin, Kirill V. ;
Volkov, Valentyn S. ;
Alonso-Gonzalez, Pablo ;
Nikitin, Alexey Yu .
PHYSICAL REVIEW B, 2019, 100 (23)
[4]   Selective excitation and imaging of ultraslow phonon polaritons in thin hexagonal boron nitride crystals [J].
Ambrosio, Antonio ;
Tamagnone, Michele ;
Chaudhary, Kundan ;
Jauregui, Luis A. ;
Kim, Philip ;
Wilson, William L. ;
Capasso, Federico .
LIGHT-SCIENCE & APPLICATIONS, 2018, 7
[5]   Interference n edge-scattering from monocrystalline gold flakes [J].
Boroviks, Sergejs ;
Wolff, Christian ;
Linnet, Jes ;
Yang, Yuanqing ;
Todisco, Francesco ;
Roberts, Alexander S. ;
Bozhevolnyi, Sergey, I ;
Hecht, Bert ;
Mortensen, N. Asger .
OPTICAL MATERIALS EXPRESS, 2018, 8 (12) :3688-3697
[6]   SYNTHESIS OF THIOL-DERIVATIZED GOLD NANOPARTICLES IN A 2-PHASE LIQUID-LIQUID SYSTEM [J].
BRUST, M ;
WALKER, M ;
BETHELL, D ;
SCHIFFRIN, DJ ;
WHYMAN, R .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1994, (07) :801-802
[7]   Real-space observation of vibrational strong coupling between propagating phonon polaritons and organic molecules [J].
Bylinkin, Andrei ;
Schnell, Martin ;
Autore, Marta ;
Calavalle, Francesco ;
Li, Peining ;
Taboada-Gutierrez, Javier ;
Liu, Song ;
Edgar, James H. ;
Casanova, Felix ;
Hueso, Luis E. ;
Alonso-Gonzalez, Pablo ;
Nikitin, Alexey Y. ;
Hillenbrand, Rainer .
NATURE PHOTONICS, 2021, 15 (03) :197-202
[8]   Sub-diffractional volume-confined polaritons in the natural hyperbolic material hexagonal boron nitride [J].
Caldwell, Joshua D. ;
Kretinin, Andrey V. ;
Chen, Yiguo ;
Giannini, Vincenzo ;
Fogler, Michael M. ;
Francescato, Yan ;
Ellis, Chase T. ;
Tischler, Joseph G. ;
Woods, Colin R. ;
Giles, Alexander J. ;
Hong, Minghui ;
Watanabe, Kenji ;
Taniguchi, Takashi ;
Maier, Stefan A. ;
Novoselov, Kostya S. .
NATURE COMMUNICATIONS, 2014, 5
[9]   Modern Scattering-Type Scanning Near-Field Optical Microscopy for Advanced Material Research [J].
Chen, Xinzhong ;
Hu, Debo ;
Mescall, Ryan ;
You, Guanjun ;
Basov, D. N. ;
Dai, Qing ;
Liu, Mengkun .
ADVANCED MATERIALS, 2019, 31 (24)
[10]   Subdiffractional focusing and guiding of polaritonic rays in a natural hyperbolic material [J].
Dai, S. ;
Ma, Q. ;
Andersen, T. ;
Mcleod, A. S. ;
Fei, Z. ;
Liu, M. K. ;
Wagner, M. ;
Watanabe, K. ;
Taniguchi, T. ;
Thiemens, M. ;
Keilmann, F. ;
Jarillo-Herrero, P. ;
Fogler, M. M. ;
Basov, D. N. .
NATURE COMMUNICATIONS, 2015, 6