In-situ investigation of hydrogen diffusion in Zircaloy-4 by means of neutron radiography

被引:19
|
作者
Grosse, M. [1 ]
van den Berg, M. [1 ,2 ]
Goulet, C. [1 ,3 ]
Kaestner, A. [4 ]
机构
[1] Karlsruhe Inst Technol, Inst Appl Mat, POB 3640, D-76021 Karlsruhe, Germany
[2] Fontys Hogsch, NL-5612 MA Eindhoven, Netherlands
[3] INSA Univ, F-31077 Toulouse 4, France
[4] PSI, Dept Spallat Source, CH-5232 Villigen, Switzerland
关键词
ZIRCONIUM ALLOYS;
D O I
10.1088/1742-6596/340/1/012106
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The hydrogen diffusion from the gas phase into Zircaloy-4 solid cylinders was investigated at various temperatures between 823 and 1473 K. Diffusion coefficients were fitted using axial hydrogen distributions for all temperatures investigated. The activation energy of the hydrogen diffusion was calculated for temperatures at which the bcc beta phase is stable. The determined value of 48.3 kJ mol(-1) K-1 is significantly higher than values published by other authors. At lower temperatures the hydrogen uptake is connected with a phase transformation from the hcp alpha- to the bcc beta-phase. The spatial phase distribution and the hydrogen concentrations in the two phases were analysed.
引用
收藏
页数:8
相关论文
共 50 条
  • [31] Electrochemical behavior of hydrogen precipitated Zircaloy-4
    Rafique, Mohsin
    Afzal, Naveed
    Deen, K. M.
    Kim, Yong-Soo
    MODERN PHYSICS LETTERS B, 2015, 29 (32):
  • [32] EFFECT OF HYDROGEN ON MECHANICAL PROPERTIES OF ZIRCALOY-4
    JOHNSON, CR
    LOWE, AL
    TRANSACTIONS OF THE AMERICAN NUCLEAR SOCIETY, 1967, 10 (02): : 465 - &
  • [33] PRECIPITATE STABILITY IN NEUTRON-IRRADIATED ZIRCALOY-4
    YANG, WJS
    JOURNAL OF NUCLEAR MATERIALS, 1988, 158 : 71 - 80
  • [34] In situ crack growth observation and fracture toughness measurement of hydrogen charged Zircaloy-4
    Bertolino, G
    Meyer, G
    Ipiña, JP
    JOURNAL OF NUCLEAR MATERIALS, 2003, 322 (01) : 57 - 65
  • [35] Effect of external stress on deuteride (hydride) precipitation in Zircaloy-4 using in situ neutron diffraction
    Lin, Jun-li
    An, Ke
    Stoica, Alexandru D.
    Heuser, Brent J.
    JOURNAL OF NUCLEAR MATERIALS, 2017, 487 : 396 - 405
  • [36] Mechanisms of Hydride Reorientation in Zircaloy-4 Studied in Situ
    Colas, Kimberly
    Motta, Arthur
    Daymond, Mark R.
    Almer, Jonathan
    ZIRCONIUM IN THE NUCLEAR INDUSTRY, 2015, 1543 : 1107 - 1137
  • [37] Neutron radiography and tomography investigations of the secondary hydriding of zircaloy-4 during simulated loss of coolant nuclear accidents
    Grosse, Mirco K.
    Stuckert, Juri
    Steinbrueck, Martin
    Kaestner, Anders P.
    Hartmann, Stefan
    7TH INTERNATIONAL TOPICAL MEETING ON NEUTRON RADIOGRAPHY (ITMNR-7), 2013, 43 : 294 - 306
  • [38] Effect of neutron beamline irradiation on hydrogen equilibrium vapor pressure over hydrided Zircaloy-4
    Luscher, W. G.
    Geelhood, K. J.
    Zipperer, T. J.
    Goodrich, S. S.
    Choi, E.
    Hines, C. C.
    Bennett, H. L.
    ANNALS OF NUCLEAR ENERGY, 2024, 208
  • [39] INVESTIGATION OF DIFFUSION-BONDING BETWEEN ZIRCALOY-4 AND 304 STAINLESS-STEEL
    SHAABAN, HI
    HAMMAD, FH
    BARON, JL
    JOURNAL OF NUCLEAR MATERIALS, 1978, 71 (02) : 277 - 285
  • [40] A comparative investigation of neutron and gamma radiation interaction properties of zircaloy-2 and zircaloy-4 with consideration of mechanical properties
    Sen Baykal, Duygu
    OPEN PHYSICS, 2024, 22 (01):