Catalytic motors for transport of colloidal cargo

被引:322
作者
Sundararajan, Shakuntala [2 ]
Lammert, Paul E. [1 ]
Zudans, Andrew W. [2 ]
Crespi, Vincent H. [1 ]
Sen, Ayusman [2 ]
机构
[1] Penn State Univ, Dept Phys, University Pk, PA 16802 USA
[2] Penn State Univ, Dept Chem, University Pk, PA 16802 USA
基金
美国国家科学基金会;
关键词
D O I
10.1021/nl072275j
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Autonomous micro- and nanomotors should, in principle, deliver materials in a site-directed fashion, powering the assembly of dynamic, nonequilibrium superstructures. Here we demonstrate that catalytic Pt-Au nanomotors can transport a prototypical cargo: polystyrene microspheres. In addition, motors with NI segments can overcome both Brownian orientational fluctuations and biased rotation of the rod-sphere doublet to enable persistent steerable uniaxial motion in an external magnetic field. Assuming a cargo-independent motive force, the speeds are inversely proportional to the Stokes resistance, which we compute using a completed double-layer boundary integral equation. In addition, we demonstrate motors transporting cargo via chemotaxis toward a H2O2 fuel source.
引用
收藏
页码:1271 / 1276
页数:6
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