Soft Photocatalysis: Organic Polymers for Solar Fuel Productions

被引：212

作者：

Vyas, Vijay S. ^{[1
]}

Lau, Vincent Wing-hei ^{[1
]}

Lotsch, Bettina V. ^{[1
,2
,3
,4
]}

机构：

[1] Max Planck Inst Solid State Res, Heisenbergstr 1, D-70569 Stuttgart, Germany

[2] Univ Munich LMU, Dept Chem, Butenandtstr 5-13, D-81377 Munich, Germany

[3] Nanosyst Initiat Munich, Schellingstr 4, D-80799 Munich, Germany

[4] Ctr NanoSci, Schellingstr 4, D-80799 Munich, Germany

来源：

CHEMISTRY OF MATERIALS | 2016年 / 28卷 / 15期

关键词：

GRAPHITIC CARBON NITRIDE; TRIAZINE-BASED FRAMEWORKS; DRIVEN HYDROGEN EVOLUTION; MOLECULAR-SYSTEMS; COVALENT; LIGHT; WATER; CRYSTALLINE; EFFICIENT; REDUCTION;

D O I：

10.1021/acs.chemmater.6b01894

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Solar fuel generation has attracted vast research interest as an environmentally benign means of producing energy from sunlight for catering to the ever growing world energy demands. As an alternative to inorganic semiconductors, organic polymers have entered the stage as promising photocatalytic systems offering a yet unprecedented scope for molecular engineering and precise tuning of optoelectronic properties. This perspective presents an overview of the development, state-of-the-art, and growth perspectives of this emerging field and highlights recent advances in photocatalyst design with a particular focus on structure property-activity relationships in structurally well-defined 2D polymers for hydrogen evolution.

引用

页码：5191 / 5204

页数：14

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