CFD analysis of a PEM fuel cell for liquid dispersion at the Interface of GDL-GFC

被引:8
作者
Hasan, A. B. Mahmud [1 ,2 ]
Wahab, M. A. [3 ]
Guo, S. M. [3 ]
机构
[1] Virginia Tech, Dept Mech Engn, Blacksburg, VA 24061 USA
[2] Univ Pittsburgh, Mech Engn & Mat Sci Dept, Pittsburgh, PA USA
[3] Louisiana State Univ, Dept Mech Engn, Baton Rouge, LA 70803 USA
关键词
Water dispersions; PEMFC; Saturation; Gas flow; Diffusion; Fluid dynamics;
D O I
10.1108/09615531111162792
中图分类号
O414.1 [热力学];
学科分类号
摘要
Purpose - The purpose of this paper is to present the results of analysis of the transport gases and liquid water between the gas diffusion layer (GDL) and gas flow channel (GFC) of proton exchange membrane fuel cells (PEMFCs). These results are then used to describe the effects of the GDL-GFC interfacial conditions on the general performance of PEMFCs. Design/methodology/approach - This analysis utilizes finite element analysis commercial codes to illustrate the transport of fluids. The gas transport data obtained from the solution are compared with the established works of others. The liquid transport processes are modeled using the Darcy equation coupled with a saturation-capillary pressure function (the Leverett function) and assuming no phase change. In addition, the boundary conditions for the liquid transport equation are varied in order to show the extent of non-uniformities at the GDL-GFC interface. Findings - Analysis shows that water dispersion from the GDL-GFC interface extends across the GDL to its other side, and eventually reduces the performance of the PEMFC. Research limitations/implications - It is well known that CFD simulation of fuel cells is, in general, still facing significant challenges due to the limited understanding of the complex physical and chemical processes existing within the fuel cell. The model is now under further development to improve its capabilities and undergoing further validations. Practical implications - The simulations can provide detailed information on some of the key fluid dynamics, physical and chemical/electro-chemical processes that exist in liquid dispersion at the interface of GDL-GFC in fuel cells which are critical for fuel cell design and optimization. Originality/value - The simulation can be used to understand liquid dispersion at the interface of GDL-GFC and provide and alternative to experimental investigations in order to improve the performance of fuel cell.
引用
收藏
页码:810 / 821
页数:12
相关论文
共 14 条
[1]   Simplified models for predicting the onset of liquid water droplet instability at the gas diffusion layer/gas flow channel interface [J].
Chen, KS ;
Hickner, MA ;
Noble, DR .
INTERNATIONAL JOURNAL OF ENERGY RESEARCH, 2005, 29 (12) :1113-1132
[2]  
Coppo M., 2005, THESIS POLITECNICO T
[3]  
Guo S.M., 2009, ASME J FUEL CELL SCI, V6
[4]  
Hasan A.B.M, 2005, THESIS LSU
[5]   Two-dimensional simulation of water transport in polymer electrolyte fuel cells [J].
Hsing, IM ;
Futerko, P .
CHEMICAL ENGINEERING SCIENCE, 2000, 55 (19) :4209-4218
[6]   Quasi-3D modeling of water transport in polymer electrolyte fuel cells [J].
Kulikovsky, AA .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2003, 150 (11) :A1432-A1439
[7]   Effects of cathode humidification on the gas-liquid interface location in a PEM fuel cell [J].
Lee, Chun-I ;
Chu, Hsin-Sen .
JOURNAL OF POWER SOURCES, 2006, 161 (02) :949-956
[8]   Effective diffusivity and water-saturation distribution in single- and two-layer PEMFC diffusion medium [J].
Nam, JH ;
Kaviany, M .
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2003, 46 (24) :4595-4611
[9]  
O'Hayre R., 2005, FUEL CELL FUNDAMENTA
[10]   LOCALIZATION OF PLATINUM IN LOW CATALYST LOADING ELECTRODES TO ATTAIN HIGH-POWER DENSITIES IN SPE FUEL-CELLS [J].
TICIANELLI, EA ;
DEROUIN, CR ;
SRINIVASAN, S .
JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 1988, 251 (02) :275-295