Plasmon Resonances of Highly Doped Two-Dimensional MoS2

被引:154
作者
Wang, Yichao [1 ]
Ou, Jian Zhen [1 ]
Chrimes, Adam F. [1 ]
Carey, Benjamin J. [1 ]
Daeneke, Torben [1 ]
Alsaif, Manal M. Y. A. [1 ]
Mortazavi, Majid [2 ]
Zhuiykov, Serge [3 ]
Medhekar, Nikhil [2 ]
Bhaskaran, Madhu [1 ]
Friend, James R. [1 ,4 ]
Strano, Michael S. [5 ]
Kalantar-Zadeh, Kourosh [1 ]
机构
[1] RMIT Univ, Sch Elect & Comp Engn, Melbourne, Vic 3000, Australia
[2] Monash Univ, Dept Mat Engn, Clayton, Vic 3800, Australia
[3] CSIRO, Div Mat Sci & Technol, Highett, Vic 3190, Australia
[4] Univ Calif San Diego, Dept Mech & Aerosp Engn, San Diego, CA 92093 USA
[5] MIT, Dept Chem Engn, Cambridge, MA 02139 USA
基金
澳大利亚研究理事会;
关键词
Two-dimensional; MoS2; plasmonics; doping; electrochemical intercalation; biosensor; ELECTRON-ENERGY-LOSS; MOLYBDENUM; PHOTOLUMINESCENCE; EXFOLIATION; CHEMISTRY; EVOLUTION; PLATFORM; LITHIUM;
D O I
10.1021/nl503563g
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The exhibition of plasmon resonances in two-dimensional (2D) semiconductor compounds is desirable for many applications. Here, by electrochemically intercalating lithium into 2D molybdenum disulfide (MoS2) nanoflakes, plasmon resonances in the visible and near UV wavelength ranges are achieved. These plasmon resonances are controlled by the high doping level of the nanoflakes after the intercalation, producing two distinct resonance peak areas based on the crystal arrangements. The system is also benchmarked for biosensing using bovine serum albumin. This work provides a foundation for developing future 2D MoS2 based biological and optical units.
引用
收藏
页码:883 / 890
页数:8
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