In the changing times and society, the problem of human psychological imbalance has become an important issue in contemporary Chinese society. At the same time, the rapid development of time and space and the complexity and changeability of human nature make view for people more the value of ideological and political education. Therefore, the psychological adjustment of ideological and political education has important practical significance. Psychological adjustment function of ideological and political education includes attitude adjustment function, emotional adjustment function and crisis adjustment function. Each adjustment function has theoretical origin of psychology and practical value of ideological and political education. Guiding ideological and political education with psychological theory and standardizing the functions, methods and paths of psychological adjustment of ideological and political education will help to improve the methodology of ideological and political education.