Investigation of high-performance perovskite nanocrystals for inkjet-printed color conversion layers with superior color purity

被引:25
作者
Lee, Sang Yoon [1 ,2 ]
Lee, Geonho [1 ,3 ]
Kim, Do Yeob [4 ]
Jang, Seong Hyun [1 ,2 ]
Choi, In [5 ]
Park, Jongwook [3 ]
Park, Hyung-Ki [6 ]
Jung, Jae Woong [2 ]
Cho, Kwan Hyun [4 ]
Choi, Jun [1 ]
机构
[1] Korea Inst Ind Technol KITECH, Human Convergence Technol R&D Dept, Ansan 15588, South Korea
[2] Kyung Hee Univ, Dept Adv Mat Engn Informat & Elect, Yongin 17104, South Korea
[3] Kyung Hee Univ, Dept Chem Engn, Yongin 17104, South Korea
[4] Korea Inst Ind Technol KITECH, Mfg Proc Platform R&D Dept, Ansan 15588, South Korea
[5] Hanyang Univ, Dept Chem Engn, Seoul 04763, South Korea
[6] Korea Inst Ind Technol KITECH, Funct Mat & Components R&D Grp, Kangnung 25440, South Korea
基金
新加坡国家研究基金会;
关键词
STABILITY; FILM;
D O I
10.1063/5.0044284
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We synthesized cesium lead-halide perovskite colloidal nanocrystals using the hot injection method for wide-color-gamut low-cost displays. An efficient surface defect passivation technique was applied to further improve the optical performance of the green and red perovskite nanocrystals. The prepared perovskite nanocrystal solutions were formulated into inkjet printable homogeneous inks and uniformly printed on the substrate with appropriate surface control. They formed the wide-color-gamut color conversion layers of quantum dot organic light-emitting diode displays. We confirmed the excellent photophysical properties of the synthesized green/red perovskite nanocrystals and the inkjet printed color conversion layers with a photoluminescence quantum yield of 99.7%/96.2% and a wide color reproduction range of 117%.
引用
收藏
页数:11
相关论文
共 31 条
[21]   Perovskites for Next-Generation Optical Sources [J].
Quan, Li Na ;
Rand, Barry P. ;
Friend, Richard H. ;
Mhaisalkar, Subodh Gautam ;
Lee, Tae-Woo ;
Sargent, Edward H. .
CHEMICAL REVIEWS, 2019, 119 (12) :7444-7477
[22]   Metal Halide Perovskite Nanocrystals: Synthesis, Post-Synthesis Modifications, and Their Optical Properties [J].
Shamsi, Javad ;
Urban, Alexander S. ;
Imran, Muhammad ;
De Trizio, Luca ;
Manna, Liberato .
CHEMICAL REVIEWS, 2019, 119 (05) :3296-3348
[23]   Highly Luminescent Cesium Lead Halide Perovskite Nanocrystals with Tunable Composition and Thickness by Ultrasonication [J].
Tong, Yu ;
Bladt, Eva ;
Aygueler, Meltem F. ;
Manzi, Aurora ;
Milowska, Karolina Z. ;
Hintermayr, Verena A. ;
Docampo, Pablo ;
Bals, Sara ;
Urban, Alexander S. ;
Polavarapu, Lakshminarayana ;
Feldmann, Jochen .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2016, 55 (44) :13887-13892
[24]   Highly Efficient CsPbBr3 Planar Perovskite Solar Cells via Additive Engineering with NH4SCN [J].
Wang, Deng ;
Li, Wenjing ;
Du, Zhenbo ;
Li, Guodong ;
Sun, Weihai ;
Wu, Jihuai ;
Lan, Zhang .
ACS APPLIED MATERIALS & INTERFACES, 2020, 12 (09) :10579-10587
[25]   Growth of ultrasmooth octadecyltrichlorosilane self-assembled monolayers on SiO2 [J].
Wang, YL ;
Lieberman, M .
LANGMUIR, 2003, 19 (04) :1159-1167
[26]   Air-stable all-inorganic perovskite quantum dot inks for multicolor patterns and white LEDs [J].
Wu Zhihai ;
Wei Jiao ;
Sun Yanni ;
Wu Jun ;
Hou Yafei ;
Wang Pan ;
Wang Nengping ;
Zhao Zhenfu .
JOURNAL OF MATERIALS SCIENCE, 2019, 54 (09) :6917-6929
[27]   Inkjet-Printed Quantum Dot Color Conversion Films for High-Resolution and Full-Color Micro Light-Emitting Diode Displays [J].
Xuan, Tongtong ;
Shi, Shuchen ;
Wang, Le ;
Kuo, Hao-Chung ;
Xie, Rong-Jun .
JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2020, 11 (13) :5184-5191
[28]   Surface Halogen Compensation for Robust Performance Enhancements of CsPbX3 Perovskite Quantum Dots [J].
Yang, Dandan ;
Li, Xiaoming ;
Wu, Ye ;
Wei, Changting ;
Qin, Zhengyuan ;
Zhang, Chunfeng ;
Sun, Zhiguo ;
Li, Yuelei ;
Wang, Yue ;
Zeng, Haibo .
ADVANCED OPTICAL MATERIALS, 2019, 7 (11)
[29]   Highly Luminescent Cesium Lead Halide Perovskite Nanocrystals Stabilized in Glasses for Light-Emitting Applications [J].
Ye, Ying ;
Zhang, Wenchao ;
Zhao, Zhiyong ;
Wang, Jing ;
Liu, Chao ;
Deng, Zhao ;
Zhao, Xiujian ;
Han, Jianjun .
ADVANCED OPTICAL MATERIALS, 2019, 7 (09)
[30]   In Situ Synthesis of Ultrastable CsPbBr3 Perovskite Nanocrystals Coated with Polyimide in a CSTR System [J].
Zhang, Jibin ;
Jiang, Pengfei ;
Wang, Yao ;
Liu, Xiangfu ;
Ma, Jinming ;
Tu, Guoli .
ACS APPLIED MATERIALS & INTERFACES, 2020, 12 (02) :3080-3085