Influence of MgO and ZrO2 buffer layers on dielectric properties of Ba(Zr0.20Ti0.80)O3 thin films prepared by sol-gel processing

被引:8
作者
Gao, L. N. [1 ]
Zhai, J. W. [1 ]
Yao, X. [1 ]
机构
[1] Tongji Univ, Funct Mat Res Lab, Shanghai Key Lab Special Artificial Microstruct M, Dept Phys, Shanghai 200092, Peoples R China
基金
中国博士后科学基金;
关键词
Thin film; Sol-gel; Dielectric properties; Orientation; Tunability; ORIENTATION; TUNABILITY; TA2O5; TIO2;
D O I
10.1016/j.apsusc.2010.10.132
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Ba(Zr0.20Ti0.80)O-3 (BZT) thin films are deposited on Pt(1 1 1)/Ti/SiO2/Si, MgO and ZrO2 buffered Pt(1 1 1)/Ti/SiO2/Si substrates by a sol-gel process. The BZT thin films directly grown on Pt(1 1 1)/Ti/SiO2/Si substrates exhibit highly (1 1 1) preferred orientation, while the films deposited on Pt(1 1 1)/Ti/SiO2/Si substrates with MgO and ZrO2 buffer layers show highly (1 1 0) preferred orientation. At 100 kHz, dielectric constants are 417, 311 and 321 for the BZT thin films grown on Pt(1 1 1)/Ti/SiO2/Si, MgO and ZrO2 buffered Pt(1 1 1)/Ti/SiO2/Si substrates, respectively. The difference in dielectric properties of three BZT films can be attributed to the series capacitance effect, interface conditions and their orientations. (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:3836 / 3839
页数:4
相关论文
共 27 条
[1]   Compositionally graded BaxSr1-xTiO3 thin films for tunable microwave applications [J].
Adikary, SU ;
Chan, HLW .
MATERIALS CHEMISTRY AND PHYSICS, 2003, 79 (2-3) :157-160
[2]   Dielectric properties and relaxor behavior of rare-earth (La, Sm, Eu, Dy, Y) substituted barium zirconium titanate ceramics [J].
Chou, Xiujian ;
Zhai, Jiwei ;
Jiang, Haitao ;
Yao, Xi .
JOURNAL OF APPLIED PHYSICS, 2007, 102 (08)
[3]  
Das SR, 2003, MATER RES SOC SYMP P, V748, P429
[4]   Investigations on the sol-gel-derived barium zirconium titanate thin films [J].
Dixit, A ;
Majumder, SB ;
Savvinov, A ;
Katiyar, RS ;
Guo, R ;
Bhalla, AS .
MATERIALS LETTERS, 2002, 56 (06) :933-940
[5]   Effects of buffer layers on the orientation and dielectric properties of Ba(Zr0.20Ti0.80)O3 thin films prepared by sol-gel method [J].
Gao, L. N. ;
Song, S. N. ;
Zhai, J. W. ;
Yao, X. ;
Xu, Z. K. .
JOURNAL OF CRYSTAL GROWTH, 2008, 310 (06) :1245-1249
[6]   Influence of rare-earth addition on dielectric properties and relaxor behavior of barium zirconium titanate thin films [J].
Gao, Lina ;
Zhai, Jiwei ;
Zhang, Yewen ;
Yao, Xi .
JOURNAL OF APPLIED PHYSICS, 2010, 107 (06)
[7]   Effects of CeO2 buffer layer thickness on the orientation and dielectric proper-ties of Ba(Zr0.20Ti0.80)O3 thin films [J].
Gao, Lina ;
Zhai, Jiwei ;
Song, Sangnian ;
Hao, Xihong ;
Yao, Xi .
JOURNAL OF CRYSTAL GROWTH, 2009, 311 (02) :299-303
[8]   A comparative study on the electrical conduction mechanisms of (Ba0.5Sr0.5)TiO3 thin films on Pt and IrO2 electrodes [J].
Hwang, CS ;
Lee, BT ;
Kang, CS ;
Kim, JW ;
Lee, KH ;
Cho, HJ ;
Horii, H ;
Kim, WD ;
Lee, SI ;
Roh, YB ;
Lee, MY .
JOURNAL OF APPLIED PHYSICS, 1998, 83 (07) :3703-3713
[9]   Dielectric properties of epitaxial Ba0.6Sr0.4TiO3 films on SiO2/Si using biaxially oriented ion-beam-assisted-deposited MgO as templates [J].
Kang, BS ;
Lee, JS ;
Stan, L ;
Lee, JK ;
DePaula, RF ;
Arendt, PN ;
Nastasi, M ;
Jia, QX .
APPLIED PHYSICS LETTERS, 2004, 85 (20) :4702-4704
[10]   High tunability (Ba,Sr)TiO3 thin films grown on atomic layer deposited TiO2 and Ta2O5 buffer layers [J].
Kim, ID ;
Tuller, HL ;
Kim, HS ;
Park, JS .
APPLIED PHYSICS LETTERS, 2004, 85 (20) :4705-4707