Nonlinear Fano interferences in open quantum systems: An exactly solvable model

被引:11
作者
Finkelstein-Shapiro, Daniel [1 ,2 ,3 ]
Calatayud, Monica [2 ,3 ,4 ]
Atabek, Osman [5 ]
Mujica, Vladimiro [1 ]
Keller, Arne [5 ]
机构
[1] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85282 USA
[2] Univ Paris 06, Sorbonne Univ, UMR 7616, Lab Chime Theor, F-75005 Paris, France
[3] CNRS, UMR 7616, Lab Chime Theor, F-75005 Paris, France
[4] Inst Univ France, Paris, France
[5] Univ Paris Saclay, Univ Paris 11, CNRS, Inst Sci Mol Orsay,UMR8214, Batiment 350, F-91405 Orsay, France
基金
美国国家科学基金会;
关键词
DYNAMICAL SEMIGROUPS; SPECTROSCOPY; RELAXATION; RESONANCE; DOTS; SCATTERING; INJECTION; STATES; PHASE;
D O I
10.1103/PhysRevA.93.063414
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We obtain an explicit solution for the stationary-state populations of a dissipative Fano model, where a discrete excited state is coupled to a continuum set of states; both excited sets of states are reachable by photoexcitation from the ground state. The dissipative dynamic is described by a Liouville equation in Lindblad form and the field intensity can take arbitrary values within the model. We show that the population of the continuum states as a function of laser frequency can always be expressed as a Fano profile plus a Lorentzian function with effective parameters whose explicit expressions are given in the case of a closed system coupled to a bath as well as for the original Fano scattering framework. Although the solution is intricate, it can be elegantly expressed as a linear transformation of the kernel of a 4 x 4 matrix which has the meaning of an effective Liouvillian. We unveil key notable processes related to the optical nonlinearity and which had not been reported to date: electromagnetic-induced transparency, population inversions, power narrowing and broadening, as well as an effective reduction of the Fano asymmetry parameter.
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页数:8
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[41]   Quantum theory of the nonlinear Fano effect in hybrid metal-semiconductor nanostructures: The case of strong nonlinearity [J].
Zhang, Wei ;
Govorov, Alexander O. .
PHYSICAL REVIEW B, 2011, 84 (08)