Effect of Gold Nanoparticles on the Crystallization and Optical Properties of Glass in ZnO-MgO-Al2O3-SiO2 System

被引：18

作者：

Shakhgildyan, Georgiy ^{[1
]}

Durymanov, Veniamin ^{[2
]}

Ziyatdinova, Mariam ^{[1
,3
]}

Atroshchenko, Grigoriy ^{[1
]}

Golubev, Nikita ^{[1
]}

Trifonov, Alexey ^{[4
,5
]}

Chereuta, Olga ^{[1
]}

Avakyan, Leon ^{[2
]}

Bugaev, Lusegen ^{[2
]}

Sigaev, Vladimir ^{[1
]}

机构：

[1] Mendeleev Univ Chem Technol, Dept Glass & Glass Ceram, Miusskaya Sq 9, Moscow 125047, Russia

[2] Southern Fed Univ, Dept Phys, Zorge St 5, Rostov Na Donu 344090, Russia

[3] Russian Acad Sci, PN Lebedev Phys Inst, Leninskiy Av 53, Moscow 119333, Russia

[4] Natl Res Univ Elect Technol MIET, Inst Phys & Appl Math, Shokin Sq,Bld 1, Moscow 124498, Russia

[5] Sci Res Inst Phys Problems, Pass 4806,Bld 6, Moscow 124498, Russia

来源：

CRYSTALS | 2022年 / 12卷 / 02期

关键词：

glass-ceramics; phase separation; nucleation; crystallization; microstructure; gahnite; gold nanoparticles; surface plasmon resonance; plasmonics; PHOSPHATE-GLASS; LUMINESCENCE; CERAMICS; MICROSTRUCTURE; SILVER; ENHANCEMENT; SCATTERING;

D O I：

10.3390/cryst12020287

中图分类号：

O7 [晶体学];

学科分类号：

0702 ; 070205 ; 0703 ; 080501 ;

摘要：

Gold nanoparticles precipitated in transparent glass-ceramics could pave the way for the development of multifunctional materials that are in demand in modern photonics and optics. In this work, we explored the effect of gold nanoparticles on the crystallization, microstructure, and optical properties of ZnO-MgO-Al2O3-SiO2 glass containing TiO2 and ZrO2 as nucleating agents. X-ray diffraction, transmission electron microscopy, Raman, and optical spectroscopy were used for the study. We showed that gold nanoparticles have no effect on the formation of gahnite nanocrystals during the glass heat treatments, while optical properties of the glass-ceramics are strongly dependent on the gold addition. A computational model was developed to predict optical properties of glass during the crystallization, and the possibility for adjusting the localized surface plasmon resonance band position with the heat treatment temperature was shown.

引用

页数：15

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