Characteristics of organic matter in PM2.5 from an e-waste dismantling area in Taizhou, China

被引:73
作者
Gu, Zeping [1 ]
Feng, Jialiang [1 ]
Han, Wenliang [1 ]
Wu, Minghong [1 ]
Fu, Jiamo [1 ,2 ]
Sheng, Guoying [2 ]
机构
[1] Shanghai Univ, Inst Environm Pollut & Hlth, Shanghai, Peoples R China
[2] Chinese Acad Sci, Guangzhou Inst Geochem, Guangzhou, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
PM2.5; e-Waste; SEOC; PAHs; Taizhou; China; ELECTRONIC WASTE; PHTHALATE-ESTERS; SOURCE APPORTIONMENT; RECYCLING SITE; URBAN AREA; AEROSOL; PBDES; PCBS; PRODUCTS; ZHEJIANG;
D O I
10.1016/j.chemosphere.2010.04.078
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Solvent extractable organic compounds in PM2.5 samples collected in Taizhou, a city famous for its electrical and electronic waste (e-waste) recycling industry in Zhejiang province of China, were analyzed to identify the main emission sources based on molecular markers. Two types of plastics which were most frequently contained in the e-wastes, wires/cables and plastic blocks, were burned in the lab and the particles emitted analyzed. The concentrations of PAHs and phthalate esters at the e-waste dismantling area during our sampling periods were about two times of that at the reference urban site, indicating the high pollution level there. The high concentrations of quaterphenyl found at the dismantling area indicated that burning of plastics or polymers was an important emission source of the PAHs in the fine particles. The diagnostic analysis based on the compositions of alkanes. hopanes and other molecular markers showed that engine exhaust, biomass burning and kitchen emissions were also important emission sources at the e-waste dismantling area. Our results suggested that more effort should be paid to control the correlative emission sources such as transportation and kitchen to achieve better air quality at the e-waste dismantling area besides regulating the recycling activities. (C) 2010 Elsevier Ltd. All rights reserved.
引用
收藏
页码:800 / 806
页数:7
相关论文
共 39 条
  • [1] ARDEN P, 2006, J AIR WASTE MANAGE, V56, P709
  • [2] Extractable organic matter in PM10 from LiWan district of Guangzhou city, PR China
    Bi, XH
    Sheng, GY
    Peng, PA
    Zhang, ZQ
    Fu, HM
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2002, 300 (1-3) : 213 - 228
  • [3] Birch ME, 1998, ANALYST, V123, P851
  • [4] Characterization and source apportionment of atmospheric organic and elemental carbon during fall and winter of 2003 in Xi'an, China
    Cao, JJ
    Wu, F
    Chow, JC
    Lee, SC
    Li, Y
    Chen, SW
    An, ZS
    Fung, KK
    Watson, JG
    Zhu, CS
    Liu, SX
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2005, 5 : 3127 - 3137
  • [5] Distribution of PBDEs in air particles from an electronic waste recycling site compared with Guangzhou and Hong Kong, South China
    Deng, W. J.
    Zheng, J. S.
    Bi, X. H.
    Fu, J. M.
    Wong, M. H.
    [J]. ENVIRONMENT INTERNATIONAL, 2007, 33 (08) : 1063 - 1069
  • [6] Atmospheric levels and cytotoxicity of PAHs and heavy metals in TSP and PM2.5 at an electronic waste recycling site in southeast China
    Deng, W. J.
    Louie, P. K. K.
    Liu, W. K.
    Bi, X. H.
    Fu, J. M.
    Wong, M. H.
    [J]. ATMOSPHERIC ENVIRONMENT, 2006, 40 (36) : 6945 - 6955
  • [7] Semi-volatile secondary organic aerosol in urban atmospheres: meeting a measurement challenge
    Eatough, DJ
    Long, RW
    Modey, WK
    Eatough, NL
    [J]. ATMOSPHERIC ENVIRONMENT, 2003, 37 (9-10) : 1277 - 1292
  • [8] Characteristics of organic matter in PM2.5 in Shanghai
    Feng, Jialiang
    Chan, Chak K.
    Fang, Ming
    Hu, Min
    He, Lingyan
    Tang, Xiaoyan
    [J]. CHEMOSPHERE, 2006, 64 (08) : 1393 - 1400
  • [9] Impact of meteorology and energy structure on solvent extractable organic compounds of PM2.5 in Beijing, China
    Feng, JL
    Chan, CK
    Fang, M
    Hu, M
    He, LY
    Tang, XY
    [J]. CHEMOSPHERE, 2005, 61 (05) : 623 - 632
  • [10] Levels and distribution of organochlorine pesticides in various media in a mega-city, China
    Fu, Shan
    Cheng, Hang-Xin
    Liu, Ying-Han
    Xu, Xiao-Bai
    [J]. CHEMOSPHERE, 2009, 75 (05) : 588 - 594