Optical second-order nonlinearity of the infrared transmitting 82GeS2•18CdGa2S4 nanocrystallized chalcogenide glass

被引:29
作者
Tao, Haizheng [1 ]
Lin, Changgui [1 ]
Gu, Shaoxuan [1 ]
Jing, Chengbin [1 ]
Zhao, Xiujian [1 ]
机构
[1] Wuhan Univ Technol, Key Lab Silicate Mat Sci & Engn, Minist Educ, Wuhan 430070, Peoples R China
基金
中国国家自然科学基金;
关键词
D O I
10.1063/1.2754361
中图分类号
O59 [应用物理学];
学科分类号
摘要
The infrared (IR) transmitting nanocrystallized chalcogenide glass only containing alpha-CdGa2S4 IR nonlinear optical crystallites, which were confirmed by x-ray diffraction and Raman scattering measurements, was fabricated through the controllable nucleation and crystallization of the glass with the composition 82GeS(2)center dot 18CdGa(2)S(4) at a temperature of 325 degrees C far below the glass transition temperature (T-g:415 degrees C) for a long duration. A clear second harmonic generation (green light, 532 nm) could be observed in the transparent 82GeS(2)center dot 18CdGa(2)S(4) nanocrystallized chalcogenide glass, demonstrating the IR frequency-doubling function of the prepared nanocrystallized composite material. (c) 2007 American Institute of Physics.
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页数:3
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