Effect of quantum tunneling on the ignition and propagation of magnetic avalanches in Mn12 acetate

被引:24
作者
McHugh, S. [1 ]
Jaafar, R.
Sarachik, M. P.
Myasoedov, Y.
Finkler, A.
Shtrikman, H.
Zeldov, E.
Bagai, R.
Christou, G.
机构
[1] CUNY City Coll, Dept Phys, New York, NY 10031 USA
[2] Weizmann Inst Sci, Dept Condensed Matter Phys, IL-76100 Rehovot, Israel
[3] Univ Florida, Dept Chem, Gainesville, FL 32611 USA
来源
PHYSICAL REVIEW B | 2007年 / 76卷 / 17期
关键词
D O I
10.1103/PhysRevB.76.172410
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Using a wire heater to ignite magnetic avalanches in fixed magnetic field applied along the easy axis of single crystals of the molecular magnet Mn(12) acetate, we report fast local measurements of the temperature and time-resolved measurements of the local magnetization as a function of magnetic field. In addition to confirming maxima in the velocity of propagation, we find that avalanches trigger at a threshold temperature which exhibits pronounced minima at resonant magnetic fields, demonstrating that thermally assisted quantum tunneling plays an important role in the ignition as well as the propagation of magnetic avalanches in molecular magnets.
引用
收藏
页数:4
相关论文
共 25 条
[1]   Local measurements of magnetization in Mn12 crystals -: art. no. 144428 [J].
Avraham, N ;
Stern, A ;
Suzuki, Y ;
Mertes, KM ;
Sarachik, MP ;
Zeldov, E ;
Myasoedov, Y ;
Shtrikman, H ;
Rumberger, EM ;
Hendrickson, DN ;
Chakov, NE ;
Christou, G .
PHYSICAL REVIEW B, 2005, 72 (14)
[2]   Macroscopic quantum tunneling in molecular magnets [J].
Barbara, B ;
Thomas, L ;
Lionti, F ;
Chiorescu, I ;
Sulpice, A .
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 1999, 200 (1-3) :167-181
[3]   Magnetic quantum tunneling in the single-molecule magnet Mn12-acetate [J].
del Barco, E ;
Kent, AD ;
Hill, S ;
North, JM ;
Dalal, NS ;
Rumberger, EM ;
Hendrickson, DN ;
Chakov, N ;
Christou, G .
JOURNAL OF LOW TEMPERATURE PHYSICS, 2005, 140 (1-2) :119-174
[4]   Heat capacity anomalies induced by magnetization quantum tunneling in a Mn12O12-acetate single crystal [J].
Fominaya, F ;
Villain, J ;
Gandit, P ;
Chaussy, J ;
Caneschi, A .
PHYSICAL REVIEW LETTERS, 1997, 79 (06) :1126-1129
[5]  
Friedman J. R., 2003, EXPLORING QUANTUM CL, P179
[6]   Steps in the hysteresis loops of a high-spin molecule [J].
Friedman, JR ;
Sarachik, MP ;
Tejada, J ;
Maciejewski, J ;
Ziolo, R .
JOURNAL OF APPLIED PHYSICS, 1996, 79 (08) :6031-6033
[7]   Macroscopic measurement of resonant magnetization tunneling in high-spin molecules [J].
Friedman, JR ;
Sarachik, MP ;
Tejada, J ;
Ziolo, R .
PHYSICAL REVIEW LETTERS, 1996, 76 (20) :3830-3833
[8]  
Garanin DA, 2007, PHYS REV B, V76, DOI 10.1103/PhysRevB.76.054410
[9]   Quantum tunneling of magnetization and related phenomena in molecular materials [J].
Gatteschi, D ;
Sessoli, R .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2003, 42 (03) :268-297
[10]  
Glassman I., 1996, COMBUSTION, V3rd