Photo-induced reduction of biomass-derived 5-hydroxymethylfurfural using graphitic carbon nitride supported metal catalysts

被引：54

作者：

Guo, Yuanyuan ^{[1
]}

Chen, Jinzhu ^{[1
]}

机构：

[1] Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China

来源：

RSC ADVANCES | 2016年 / 6卷 / 104期

基金：

中国国家自然科学基金;

关键词：

VISIBLE-LIGHT; HYDROGEN-PRODUCTION; SELECTIVE HYDROGENATION; PHOTOCATALYTIC REDUCTION; MILD CONDITIONS; FACILE APPROACH; ALLOY CATALYST; WATER; G-C3N4; NANOPARTICLES;

D O I：

10.1039/c6ra19153c

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Photo-catalytic reduction of biomass-derived 5-hydroxymethylfurfural (HMF) into 2,5-dihydroxymethylfuran (DHMF) under visible light irradiation is achieved by using a platinum catalyst supported on graphitic carbon nitride (Pt/g-C3N4). Pt/g-C3N4 acts as a multifunctional and tandem catalyst to successively promote the photo-induced water splitting to form hydrogen and the successive activation of the produced hydrogen for HMF reduction, yielding DHMF yield of 6.5% with TOF of 0.457 h(-1). This research provides a sustainable and green pathway for biomass conversion using solar radiation as a driving force.

引用

页码：101968 / 101973

页数：6

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