Photo-induced reduction of biomass-derived 5-hydroxymethylfurfural using graphitic carbon nitride supported metal catalysts

被引：54
|
作者：
Guo, Yuanyuan [1 ]
Chen, Jinzhu [1 ]
机构：
[1] Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China
来源：
RSC ADVANCES | 2016年 / 6卷 / 104期
基金：
中国国家自然科学基金;
关键词：
VISIBLE-LIGHT; HYDROGEN-PRODUCTION; SELECTIVE HYDROGENATION; PHOTOCATALYTIC REDUCTION; MILD CONDITIONS; FACILE APPROACH; ALLOY CATALYST; WATER; G-C3N4; NANOPARTICLES;
D O I：
10.1039/c6ra19153c
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Photo-catalytic reduction of biomass-derived 5-hydroxymethylfurfural (HMF) into 2,5-dihydroxymethylfuran (DHMF) under visible light irradiation is achieved by using a platinum catalyst supported on graphitic carbon nitride (Pt/g-C3N4). Pt/g-C3N4 acts as a multifunctional and tandem catalyst to successively promote the photo-induced water splitting to form hydrogen and the successive activation of the produced hydrogen for HMF reduction, yielding DHMF yield of 6.5% with TOF of 0.457 h(-1). This research provides a sustainable and green pathway for biomass conversion using solar radiation as a driving force.
引用
收藏
页码：101968 / 101973
页数：6
相关论文
共 50 条
  • [21] Perovskite type oxide-supported Ni catalysts for the production of 2,5-dimethylfuran from biomass-derived 5-hydroxymethylfurfural
    Chen, Meng-Yuan
    Chen, Chu-Bai
    Zada, Bakht
    Fu, Yao
    GREEN CHEMISTRY, 2016, 18 (13) : 3858 - 3866
  • [22] Influence of Lewis and Bronsted acidic sites on graphitic carbon nitride catalyst for aqueous phase conversion of biomass derived monosaccharides to 5-hydroxymethylfurfural
    Chhabra, Tripti
    Dhingra, Suman
    Nagaraja, C. M.
    Krishnan, Venkata
    CARBON, 2021, 183 : 984 - 998
  • [23] Sulfonated graphitic carbon nitride as a highly selective and efficient heterogeneous catalyst for the conversion of biomass-derived saccharides to 5-hydroxymethylfurfural in green solvents (vol 21, pg 6012, 2019)
    Chhabra, Tripti
    Bahuguna, Ashish
    Dhankhar, Sandeep Singh
    Nagaraja, C. M.
    Krishnan, Venkata
    GREEN CHEMISTRY, 2020, 22 (02) : 563 - 563
  • [24] Optimization of Electrochemical Reduction of Biomass Derived 5-Hydroxymethylfurfural (HMF): A Volcano Plot and Bimetallic Catalysts
    Luo, Xingyu
    Xie, Cheng
    Zhao, Zhefei
    Shi, Meiqin
    Zheng, Huajun
    CHEMSUSCHEM, 2024, 17 (20)
  • [25] Pairing Electrocatalytic Reduction and Oxidation of Biomass-Derived 5-Hydroxymethylfurfural into Highly Value-Added Chemicals
    Zhang, Man
    Zheng, Zhikeng
    Zhang, Xiaodie
    Jiang, Zhiwei
    Yong, Xue
    Li, Ke
    Tu, Xin
    Yan, Kai
    JACS AU, 2025, 5 (02): : 937 - 947
  • [26] Catalytic hydrogenolysis of biomass-derived 5-hydroxymethylfurfural to biofuel 2, 5-dimethylfuran
    Wang, Xiaofeng
    Liang, Xinhua
    Li, Jiaomin
    Li, Qingbo
    APPLIED CATALYSIS A-GENERAL, 2019, 576 : 85 - 95
  • [27] State-of-the-art advances and perspectives in the separation of biomass-derived 5-hydroxymethylfurfural
    Hu, Lei
    Jiang, Yetao
    Wu, Zhen
    Wang, Xiaoyu
    He, Aiyong
    Xu, Jiaxing
    Xu, Jiming
    JOURNAL OF CLEANER PRODUCTION, 2020, 276 (276)
  • [28] Diverse Applications of Biomass-Derived 5-Hydroxymethylfurfural and Derivatives as Renewable Starting Materials
    Chacon-Huete, Franklin
    Messina, Cynthia
    Cigana, Brandon
    Forgione, Pat
    CHEMSUSCHEM, 2022, 15 (13)
  • [29] Recent advance on the catalytic system for efficient production of biomass-derived 5-hydroxymethylfurfural
    Hu, Di
    Zhang, Man
    Xu, Hong
    Wang, Yuchen
    Yan, Kai
    RENEWABLE & SUSTAINABLE ENERGY REVIEWS, 2021, 147
  • [30] A multi-walled carbon nanotube-supported acidic ionic liquid catalyst for the conversion of biomass-derived saccharides to 5-hydroxymethylfurfural
    Niakan, Mahsa
    Masteri-Farahani, Majid
    Seidi, Farzad
    Karimi, Sabah
    Shekaari, Hemayat
    REACTION CHEMISTRY & ENGINEERING, 2023, 8 (10) : 2473 - 2480
12345