Direct Synthesis of Crystalline Graphdiyne Analogue Based on Supramolecular Interactions

被引：66
作者：
Zhou, Weixiang [1 ,2 ]
Shen, Han [1 ,2 ]
Wu, Chenyu [3 ]
Tu, Zeyi [1 ,2 ]
He, Feng [1 ]
Gu, Yanan [1 ,2 ]
Xue, Yurui [1 ]
Zhao, Yingjie [3 ]
Yi, Yuanping [1 ,2 ]
Li, Yongjun [1 ,2 ]
Li, Yuliang [1 ,2 ]
机构：
[1] Chinese Acad Sci, Inst Chem, CAS Res Educ Ctr Excellence Mol Sci, BNLMS,CAS Key Lab Organ Solids, Beijing 100190, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] Qingdao Univ Sci & Technol, Coll Polymer Sci & Engn, Qingdao 266042, Peoples R China
来源：
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2019年 / 141卷 / 01期
关键词：
PERFORMANCE; GRAPHYNE; NANOWIRES; SCAFFOLDS; RAMAN;
D O I：
10.1021/jacs.8b09945
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
The synthesis of graphdiyne with an ordered internal structure is highly attractive for its various scientific and application investigations. We reported herein a rational method to fabricate a graphdiyne analogue with the help of supramolecular chemistry. The introduction of pi-pi/CH-pi interactions controlled the conformations of the precursors and afforded multilayer graphdiyne analogue Ben-GDY through the wet chemical method. The in-plane periodicity of the multilayer Ben-GDY was corroborated by transmission electron microscopy and selected area electron diffraction, which showed a pattern well matched with ABC-style stacking.
引用
收藏
页码：48 / 52
页数：5
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