An Ultrahigh-Performance Photodetector based on a Perovskite-Transition-Metal-Dichalcogenide Hybrid Structure

被引:266
作者
Kang, Dong-Ho [1 ]
Pae, Seong Ryul [2 ]
Shim, Jaewoo [1 ]
Yoo, Gwangwe [1 ]
Jeon, Jaeho [3 ]
Leem, Jung Woo [4 ]
Yu, Jae Su [5 ]
Lee, Sungjoo [3 ]
Shin, Byungha [2 ]
Park, Jin-Hong [1 ]
机构
[1] Sungkyunkwan Univ, Sch Elect & Elect Engn, Suwon 440746, South Korea
[2] Korea Adv Inst Sci & Technol KAIST, Dept Mat Sci & Engn, Daejeon 305338, South Korea
[3] Sungkyunkwan Univ, SKKU Adv Inst Nanotechnol SAINT, Suwon 440746, South Korea
[4] Purdue Univ, Weldon Sch Biomed Engn, 610 Perdue Mall, W Lafayette, IN 47907 USA
[5] Kyung Hee Univ, Dept Elect & Radio Engn, Yongin 446701, South Korea
基金
新加坡国家研究基金会;
关键词
THIN-FILM TRANSISTORS; MOS2; PHOTODETECTOR; SOLAR-CELLS; PHOTOTRANSISTORS; PHOTOLUMINESCENCE; TRANSPARENT;
D O I
10.1002/adma.201600992
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
An ultrahigh performance MoS2 photodetector with high photoresponsivity (1.94 x 10(6) A W-1) and detectivity (1.29 x 10(12) Jones) under 520 nm and 4.63 pW laser exposure is demonstrated. This photodetector is based on a methylammonium lead halide perovskite/MoS2 hybrid structure with (3-aminopropyl)triethoxysilane doping. The performance degradation caused by moisture is also minimized down to 20% by adopting a new encapsulation bilayer of octadecyltrichlorosilane/polymethyl methacrylate.
引用
收藏
页码:7799 / +
页数:9
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