quantum paralectric;
thermal Hall effect;
dilute metal;
Hall angle;
phonon drag;
PHASE;
CONDUCTIVITY;
TRANSITION;
D O I:
10.1073/pnas.2201975119
中图分类号:
O [数理科学和化学];
P [天文学、地球科学];
Q [生物科学];
N [自然科学总论];
学科分类号:
07 ;
0710 ;
09 ;
摘要:
SrTiO3, a quantum paralectric, displays a detectable phonon thermalHall effect (THE). Here, we show that the amplitude of the THE is extremely sensitive to stoichiometry. It drastically decreases upon substitution of a tiny fraction of Sr atoms with Ca, which stabilizes the ferroelectric order. It drastically increases by an even lower density of oxygen vacancies, which turn the system to a dilute metal. The enhancement in the metallic state exceeds by far the sum of the electronic and the phononic contributions. We explain this observation as an outcome of three features: 1) Heat is mostly transported by phonons; 2) the electronic Hall angle is extremely large; and 3) there is substantial momentum exchange between electrons and phonons. Starting from Herring's picture of phonon drag, we arrive to a quantitative account of the enhanced THE. Thus, phonon drag, hitherto detected as an amplifier of thermoelectric coefficients, can generate a purely thermal transverse response in a dilute metal with a large Hall angle. Our results reveal a hitherto-unknown consequence of momentum-conserving collisions between electrons and phonons.
机构:
Max Planck Inst Solid State Res, Stuttgart, GermanyMax Planck Inst Solid State Res, Stuttgart, Germany
Bruin, J. A. N.
Claus, R. R.
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机构:
Max Planck Inst Solid State Res, Stuttgart, GermanyMax Planck Inst Solid State Res, Stuttgart, Germany
Claus, R. R.
Matsumoto, Y.
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机构:
Max Planck Inst Solid State Res, Stuttgart, GermanyMax Planck Inst Solid State Res, Stuttgart, Germany
Matsumoto, Y.
Kurita, N.
论文数: 0引用数: 0
h-index: 0
机构:
Tokyo Inst Technol, Dept Phys, Tokyo, JapanMax Planck Inst Solid State Res, Stuttgart, Germany
Kurita, N.
Tanaka, H.
论文数: 0引用数: 0
h-index: 0
机构:
Tokyo Inst Technol, Dept Phys, Tokyo, JapanMax Planck Inst Solid State Res, Stuttgart, Germany
Tanaka, H.
Takagi, H.
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h-index: 0
机构:
Max Planck Inst Solid State Res, Stuttgart, Germany
Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo, JapanMax Planck Inst Solid State Res, Stuttgart, Germany
机构:
Max Planck Inst Solid State Res, Stuttgart, GermanyMax Planck Inst Solid State Res, Stuttgart, Germany
Bruin, J. A. N.
Claus, R. R.
论文数: 0引用数: 0
h-index: 0
机构:
Max Planck Inst Solid State Res, Stuttgart, GermanyMax Planck Inst Solid State Res, Stuttgart, Germany
Claus, R. R.
Matsumoto, Y.
论文数: 0引用数: 0
h-index: 0
机构:
Max Planck Inst Solid State Res, Stuttgart, GermanyMax Planck Inst Solid State Res, Stuttgart, Germany
Matsumoto, Y.
Kurita, N.
论文数: 0引用数: 0
h-index: 0
机构:
Tokyo Inst Technol, Dept Phys, Tokyo, JapanMax Planck Inst Solid State Res, Stuttgart, Germany
Kurita, N.
Tanaka, H.
论文数: 0引用数: 0
h-index: 0
机构:
Tokyo Inst Technol, Dept Phys, Tokyo, JapanMax Planck Inst Solid State Res, Stuttgart, Germany
Tanaka, H.
Takagi, H.
论文数: 0引用数: 0
h-index: 0
机构:
Max Planck Inst Solid State Res, Stuttgart, Germany
Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo, JapanMax Planck Inst Solid State Res, Stuttgart, Germany