Mesoporous S doped Fe-N-C materials as highly active oxygen reduction reaction catalyst

被引：46

作者：

Guan, Zhi ^{[1
]}

Zhang, Xuejiang ^{[1
]}

Chen, Wenxing ^{[2
]}

Pei, Jiajing ^{[1
]}

Liu, Di ^{[1
]}

Xue, Yanrong ^{[1
]}

Zhu, Wei ^{[1
]}

Zhuang, Zhongbin ^{[1
]}

机构：

[1] Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing Key Lab Energy Environm Catalysis, Beijing 100029, Peoples R China

[2] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China

来源：

CHEMICAL COMMUNICATIONS | 2018年 / 54卷 / 85期

基金：

中国国家自然科学基金;

关键词：

HIGH-PERFORMANCE ELECTROCATALYSTS; METAL-FREE ELECTROCATALYSTS; EFFICIENT ELECTROCATALYST; POROUS CARBONS; SITES; IRON; GRAPHENE; BORON; NANOSHEETS; ATOMS;

D O I：

10.1039/c8cc05273e

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Mesoporous Fe, S, N doped carbon (m-FeSNC) materials have been successfully synthesized by pyrolysis of polymerized o-phenylenediamine using binary initiators. It exhibited high electrocatalytic activity towards oxygen reduction reaction, and zinc-air battery with higher performance has been fabricated using m-FeSNC than using commercial Pt/C.

引用

页码：12073 / 12076

页数：4

共 44 条

[11] Nonprecious Metal Catalysts for Oxygen Reduction in Heterogeneous Aqueous Systems [J].

Gewirth, Andrew A. ;

Varnell, Jason A. ;

DiAscro, Angela M. .

CHEMICAL REVIEWS, 2018, 118 (05) :2313-2339

[12] EQUILIBRIUM SURFACE SEGREGATION OF DISSOLVED NONMETAL ATOMS ON IRON(100) FACES [J].

GRABKE, HJ ;

PAULITSCHKE, W ;

TAUBER, G ;

VIEFHAUS, H .

SURFACE SCIENCE, 1977, 63 (01) :377-389

[13] Role of sulphur in carburization, carbide formation and metal dusting of iron [J].

Grabke, HJ ;

Moszynski, D ;

Müller-Lorenz, EM ;

Schneider, A .

SURFACE AND INTERFACE ANALYSIS, 2002, 34 (01) :369-374

[14] NEW FUEL CELL CATHODE CATALYST [J].

JASINSKI, R .

NATURE, 1964, 201 (492) :1212-&

[15] Spectroscopic insights into the nature of active sites in iron-nitrogen-carbon electrocatalysts for oxygen reduction in acid [J].

Jia, Qingying ;

Ramaswamy, Nagappan ;

Tylus, Urszula ;

Strickland, Kara ;

Li, Jingkun ;

Serov, Alexey ;

Artyushkova, Kateryna ;

Atanassov, Plamen ;

Anibal, Jacob ;

Gumeci, Cenk ;

Barton, Scott Calabrese ;

Sougrati, Moulay-Tahar ;

Jaouen, Frederic ;

Halevi, Barr ;

Mukerjee, Sanjeev .

NANO ENERGY, 2016, 29 :65-82

[16] Cu-MOF-Derived Cu/Cu2O Nanoparticles and CuNxCy Species to Boost Oxygen Reduction Activity of Ketjenblack Carbon in Al-Air Battery [J].

Li, Jingsha ;

Zhou, Nan ;

Song, Jingya ;

Fu, Liang ;

Yan, Jun ;

Tang, Yougen ;

Wang, Haiyan .

ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2018, 6 (01) :413-421

[17] Recent advances in zinc-air batteries [J].

Li, Yanguang ;

Dai, Hongjie .

CHEMICAL SOCIETY REVIEWS, 2014, 43 (15) :5257-5275

[18] Hierarchically porous carbons with optimized nitrogen doping as highly active electrocatalysts for oxygen reduction [J].

Liang, Hai-Wei ;

Zhuang, Xiaodong ;

Bruller, Sebastian ;

Feng, Xinliang ;

Mullen, Klaus .

NATURE COMMUNICATIONS, 2014, 5

[19] Influence of Iron Source Type on the Electrocatalytic Activity toward Oxygen Reduction Reaction in Fe-N/C for Al-Air Batteries [J].

Liu, Depei ;

Fu, Liang ;

Huang, Xiaobing ;

Liu, Kun ;

Li, Jingsha ;

Xie, Hualin ;

Wang, Haiyan ;

Tang, Yougen .

JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2018, 165 (09) :F662-F670

[20] Synthesis and supercapacitor performance studies of N-doped graphene materials using o-phenylenediamine as the double-N precursor [J].

Lu, Yanhong ;

Zhang, Fan ;

Zhang, Tengfei ;

Leng, Kai ;

Zhang, Long ;

Yang, Xi ;

Ma, Yanfeng ;

Huang, Yi ;

Zhang, Mingjie ;

Chen, Yongsheng .

CARBON, 2013, 63 :508-516

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