Highly dispersed nickel anchored on a N-doped carbon molecular sieve derived from metal-organic frameworks for efficient hydrodeoxygenation in the aqueous phase

被引：24

作者：

Fan, Ruoyu ^{[1
,2
]}

Hu, Zhi ^{[1
,2
]}

Chen, Chun ^{[1
]}

Zhu, Xiaoguang ^{[1
]}

Zhang, Haimin ^{[1
]}

Zhang, Yunxia ^{[1
]}

Zhao, Huijun ^{[1
,3
]}

Wang, Guozhong ^{[1
]}

机构：

[1] Chinese Acad Sci, Inst Solid State Phys, CAS Ctr Excellence Nanosci,Key Lab Mat Phys, Anhui Key Lab Nanomat & Nanotechnol,Ctr Environm, Hefei 230031, Anhui, Peoples R China

[2] Univ Sci & Technol China, Grad Sch, Sci Isl Branch, Hefei 230026, Anhui, Peoples R China

[3] Griffith Univ, Ctr Clean Environm & Energy, Gold Coast Campus, Southport, Qld 4222, Australia

来源：

CHEMICAL COMMUNICATIONS | 2020年 / 56卷 / 49期

基金：

中国国家自然科学基金;

关键词：

SELECTIVE HYDROGENATION; NANOPARTICLES; CATALYST; CO; VANILLIN; COPPER; SITES;

D O I：

10.1039/d0cc02620d

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

ZIF-8 was employed as a template to synthesize HD-Ni/N-CMS containing highly dispersed Ni at the atomic level anchored on a N-doped carbon molecular sieve for vanillin hydrodeoxygenation. The ZIF-8 structure was inherited and Ni-N bonds were formed by the coordination of Ni with N-rich defects, therefore it exhibited a high turnover frequency (1047.1 h(-1)) and good stability.

引用

页码：6696 / 6699

页数：4

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