Air pollution inputs to the Mojave Desert by fusing surface mobile and airborne in situ and airborne and satellite remote sensing: A case study of interbasin transport with numerical model validation

被引:8
作者
Leifer, Ira [1 ]
Melton, Christopher [1 ]
Chatfield, Robert [2 ]
Cui, Xinguang [3 ]
Fischer, Marc L. [4 ]
Fladeland, Matthew [2 ]
Gore, Warren [2 ]
Hlavka, Dennis L. [5 ]
Iraci, Laura T. [2 ]
Marrero, Josette [2 ]
Ryoo, Ju-Mee [2 ]
Tanaka, Tomoaki [2 ]
Yates, Emma [2 ]
Yorks, John E. [5 ]
机构
[1] Bubbleol Res Int, Solvang, CA 93463 USA
[2] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA
[3] Huazhong Univ Sci & Technol, Luoyu Rd 1037, Wuhan, Peoples R China
[4] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA
[5] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA
关键词
Methane; Flux estimation; Airborne campaign; Air basin; Fire; Smoke; Transport; Weather regional forecast model; LiDAR; Aerosol optical depth; COMEX; RISING ASIAN EMISSIONS; AMMONIA EMISSIONS; DISCOVER-AQ; OZONE; CLIMATE; METHANE; SENSITIVITY; REGION; LAND; CO2;
D O I
10.1016/j.atmosenv.2019.117184
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Deserts are fragile and highly sensitive ecosystems that increasingly are affected by upwind urban areas and industrial activities. The Los Angeles Basin (LAB) contributes to poor air quality in downwind deserts including the Mojave Desert. Few studies have investigated potential air pollution inputs to the Mojave, whose fragile ecosystem includes endangered plant and animal species. Data were collected on 19 August 2015 by a mobile air quality laboratory, AMOG (AutoMObile trace Gas) Surveyor, that observed inputs can arise from the LAB as well as the San Joaquin Valley (SJV), California. The campaign used a strong methane (CH4) plume as a tracer for the downwind fate of emissions from Bakersfield area petroleum production and also measured ozone (O-3). Additional in situ concurrent airborne GHG and O-3 data were collected by AJAX - Alpha Jet Atmospheric eXperiment. Both AMOG and AJAX measure winds. Mojave Desert air quality was very poor (visibility 4 km). Based on the winds, an additional source was inferred beyond the LAB and SJV Basins. Numerical transport modeling and analysis of aerosol lidar data collected the same day by the Cloud Profiling LiDAR onboard the Earth Research-2 stratospheric airplane demonstrated that fires in Northern California were responsible, with prevailing winds transporting air southwards along the eastern Sierra Nevada Range (Bishop Valley) to the Mojave. Whereas the southern and eastern Mojave are impacted by SJV and LAB outflow, the north Mojave generally avoids these inputs. This study shows it can be affected by even distant wildfires, which likely will increase in occurrence and intensity from climate change. Thus, regulatory efforts to reduce air quality impacts on the endangered Mojave ecosystem must include wildfires and also account for the significant differences between different regions of the Mojave. Currently, there is a paucity of studies, highlighting the critical need for field research.
引用
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页数:13
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