High Field Optical Nonlinearity and the Kramers-Kronig Relations

被引:59
作者
Wahlstrand, J. K. [1 ]
Cheng, Y. -H. [1 ]
Milchberg, H. M. [1 ]
机构
[1] Univ Maryland, Inst Res Elect & Appl Phys, College Pk, MD 20742 USA
基金
美国国家科学基金会;
关键词
COMPRESSION; IONIZATION; PULSES; SOLIDS; ATOMS;
D O I
10.1103/PhysRevLett.109.113904
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The nonlinear optical response to high fields is absolutely measured for the noble gas atoms He, Ne, Ar, Kr, and Xe. We find that the response is quadratic in the laser field magnitude up to the ionization threshold of each gas. Its size and quadratic dependence are well predicted by a Kramers-Kronig analysis employing known ionization probabilities, and the results are consistent with calculations using the time-dependent Schrodinger equation.
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页数:5
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