Gradient HfB2-SiC multilayer oxidation resistant coating for C/C composites

被引:47
作者
Wang, Peipei [1 ]
Tong, Mingde [1 ]
Wang, Hanhui [1 ]
Li, Hejun [1 ]
Jia, Yujun [1 ]
Li, Bo [1 ]
Zhang, Yulei [1 ]
Zhao, Zhigang [1 ]
机构
[1] Northwestern Polytech Univ, Carbon Carbon Composites Res Ctr, State Key Lab Solidificat Proc, Xian 710072, Shaanxi, Peoples R China
基金
中国国家自然科学基金;
关键词
Carbon/carbon composites; Coating; Oxidation; COATED CARBON/CARBON COMPOSITES; CHEMICAL-VAPOR-DEPOSITION; HIGH-TEMPERATURE OXIDATION; THERMAL-SHOCK RESISTANCE; SILICON-CARBIDE; PACK CEMENTATION; MICROSTRUCTURE; LAYER; TRANSITION; PROTECTION;
D O I
10.1016/j.ceramint.2018.08.104
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The gradient HfB2 modified SiC coating was prepared on the surface of SiC-coated C/C composites by in-situ synthesis. Anti-oxidation behaviors of the coated C/C samples at 1773, 1873 and 1973 K were investigated. The results show that the gradient HfB2 modified SiC coatings possess excellent oxidation resistance, which can protect C/C substrates from oxidation for 800, 305 and 100 h at 1773, 1873 and 1973 K, respectively. In addition, with the oxidation temperature increasing, the evaporation of the Hf-Si-O glass layer and the active oxidation of SiC were accelerated, which is the reason for the worst oxidation resistance of the sample at 1973 K among the three temperatures.
引用
收藏
页码:20968 / 20973
页数:6
相关论文
共 34 条
[1]   Mechanical activation-assisted autoclave processing and sintering of HfB2-HfO2 ceramic powders [J].
Akcamli, Nazli ;
Agaogullari, Duygu ;
Balci, Ozge ;
Ovecoglu, M. Lutfi ;
Duman, Ismail .
CERAMICS INTERNATIONAL, 2016, 42 (13) :14642-14655
[2]   Determination of the active-to-passive transition in the oxidation of silicon carbide in standard and microwave-excited air [J].
Balat, MJH .
JOURNAL OF THE EUROPEAN CERAMIC SOCIETY, 1996, 16 (01) :55-62
[3]   Oxidation Resistance of Hafnium Diboride Ceramics with Additions of Silicon Carbide and Tungsten Boride or Tungsten Carbide [J].
Carney, Carmen M. ;
Parthasarathy, Triplicane A. ;
Cinibulk, Michael K. .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 2011, 94 (08) :2600-2607
[4]   Oxidation protection of SiC-coated C/C composites by SiC nanowire-toughened CrSi2-SiC-Si coating [J].
Chu Yanhui ;
Li Hejun ;
Fu Qiangang ;
Qi Lehua ;
Wei Bingbo .
CORROSION SCIENCE, 2012, 55 :394-400
[5]   Thermodynamic analysis of ZrB2-SiC oxidation:: Formation of a SiC-depleted region [J].
Fahrenholtz, William G. .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 2007, 90 (01) :143-148
[6]   Oxidation and ablation resistance of the ZrB2-CrSi2-Si/SiC coating for C/C composites at high temperature [J].
Feng, Tao ;
Li, Hejun ;
Hu, Manhong ;
Lin, Hongjiao ;
Li, Lu .
JOURNAL OF ALLOYS AND COMPOUNDS, 2016, 662 :302-307
[7]   Microstructure and oxidation of multi-layer MoSi2-CrSi2-Si coatings for SiC coated carbon/carbon composites [J].
Feng, Tao ;
Li, He-Jun ;
Fu, Qian-Gang ;
Shen, Xue-Tao ;
Wu, Heng .
CORROSION SCIENCE, 2010, 52 (09) :3011-3017
[8]   Silicon carbide coating to protect carbon/carbon composites against oxidation [J].
Fu, QG ;
Li, HJ ;
Shi, XH ;
Li, KZ ;
Sun, GD .
SCRIPTA MATERIALIA, 2005, 52 (09) :923-927
[9]   AMOSi2-SiC-Si/glass oxidation protective coating for carbon/carbon composites [J].
Fu Qian-Gang ;
Li He-Jun ;
Li Ke-Zhi ;
Shi Xiao-Hong ;
Huang Min .
CARBON, 2006, 44 (15) :3361-3364
[10]   Nanowire-toughened transition layer to improve the oxidation resistance of SiC-MoSi2-ZrB2 coating for C/C composites [J].
Fu, Qian-Gang ;
Jing, Jun-Yi ;
Tan, Bi-Yi ;
Yuan, Rui-Mei ;
Zhuang, Lei ;
Li, Lu .
CORROSION SCIENCE, 2016, 111 :259-266