Uniform FexNiy Nanospheres: Cost-Effective Electrocatalysts for Nonaqueous Rechargeable Li-O2` Batteries

被引:36
作者
Yuan, Mengwei [1 ,2 ]
Nan, Caiyun [1 ,2 ]
Yang, Yan [1 ,2 ]
Sun, Genban [1 ,2 ,3 ]
Li, Huifeng [1 ,2 ]
Ma, Shulan [1 ,2 ]
机构
[1] Beijing Normal Univ, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China
[2] Beijing Normal Univ, Coll Chem, Beijing 100875, Peoples R China
[3] Univ Sci & Technol Beijing, Dept Mat Phys & Chem, Beijing 100083, Peoples R China
来源
ACS OMEGA | 2017年 / 2卷 / 08期
基金
美国国家科学基金会;
关键词
LITHIUM-AIR BATTERIES; PHASE-CONTROLLED SYNTHESIS; REDUCED GRAPHENE OXIDE; HIGH-CAPACITY; EFFICIENT ELECTROCATALYSTS; CYCLING STABILITY; CATHODE MATERIALS; POROUS GRAPHENE; NANOPARTICLES; CARBON;
D O I
10.1021/acsomega.7b00497
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Uniform FexNiy nanospheres were synthesized via a simple solvothermal method and used as electrocatalysts for Li-O-2 batteries. Fe7Ni3 nanospheres exhibited relatively high catalytic activities in the electrochemical tests. They delivered a reversible capacity of more than 7000 mAh/gKB and gave a discharge-charge voltage gap reduction of 250 mV compared with Ketjen Black.
引用
收藏
页码:4269 / 4277
页数:9
相关论文
共 55 条
[1]   Graphene enhances the magnetoresistance of FeNi3 nanoparticles in hierarchical FeNi3-graphene nanocomposites [J].
Abellan, G. ;
Prima-Garcia, H. ;
Coronado, E. .
JOURNAL OF MATERIALS CHEMISTRY C, 2016, 4 (11) :2252-2258
[2]   The Role of Catalysts and Peroxide Oxidation in Lithium-Oxygen Batteries [J].
Black, Robert ;
Lee, Jin-Hyon ;
Adams, Brian ;
Mims, Charles A. ;
Nazar, Linda F. .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2013, 52 (01) :392-396
[3]  
Bruce PG, 2012, NAT MATER, V11, P19, DOI [10.1038/nmat3191, 10.1038/NMAT3191]
[4]   Hexagonal and cubic Ni nanocrystals grown on graphene: phase-controlled synthesis, characterization and their enhanced microwave absorption properties [J].
Chen, Tingting ;
Deng, Fang ;
Zhu, Jia ;
Chen, Caifeng ;
Sun, Genban ;
Ma, Shulan ;
Yang, Xiaojing .
JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (30) :15190-15197
[5]   Multi-walled carbon nanotube papers as binder-free cathodes for large capacity and reversible non-aqueous Li-O2 batteries [J].
Chen, Yong ;
Li, Fujun ;
Tang, Dai-Ming ;
Jian, Zelang ;
Liu, Chang ;
Golberg, Dmitri ;
Yamada, Atsuo ;
Zhou, Haoshen .
JOURNAL OF MATERIALS CHEMISTRY A, 2013, 1 (42) :13076-13081
[6]   Metal-air batteries: from oxygen reduction electrochemistry to cathode catalysts [J].
Cheng, Fangyi ;
Chen, Jun .
CHEMICAL SOCIETY REVIEWS, 2012, 41 (06) :2172-2192
[7]   Single layer graphene encapsulating non-precious metals as high-performance electrocatalysts for water oxidation [J].
Cui, Xiaoju ;
Ren, Pengju ;
Deng, Dehui ;
Deng, Jiao ;
Bao, Xinhe .
ENERGY & ENVIRONMENTAL SCIENCE, 2016, 9 (01) :123-129
[8]   Enhanced Cycling Stability of Hybrid Li-Air Batteries Enabled by Ordered Pd3Fe Intermetallic Electrocatalyst [J].
Cui, Zhiming ;
Li, Longjun ;
Manthiram, Arumugam ;
Goodenough, John B. .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (23) :7278-7281
[9]   RAMAN-SPECTRA OF PEROXIDES [J].
EYSEL, HH ;
THYM, S .
ZEITSCHRIFT FUR ANORGANISCHE UND ALLGEMEINE CHEMIE, 1975, 411 (02) :97-102
[10]   Critical Challenges in Rechargeable Aprotic Li-O2 Batteries [J].
Feng, Ningning ;
He, Ping ;
Zhou, Haoshen .
ADVANCED ENERGY MATERIALS, 2016, 6 (09)