We discuss the role of the dynamic glass-forming fragile-to-strong crossover (FSC) in supercooled liquids. In the FSC, significant dynamic changes such as the decoupling (the violation of the Stokes-Einstein relation) of homologous transport parameters, e. g., the density relaxation time tau and the viscosity eta, occur at a characteristic temperature T-c. We study the FSC using a scaling law approach. In particular, we use both forms of the mode-coupling theory (MCT): the original (ideal) and the extended form, which explicitly describes energy hopping processes. We demonstrate that T-c plays the most important physical role in understanding dynamic arrest processes.
机构:
Buryat State Univ, Ul Smolina 24a, Ulan Ude 670000, Russia
Russian Acad Sci, Inst Phys Mat Sci, Siberian Branch, Ul Sakhyanovoi 8, Ulan Ude 670047, RussiaBuryat State Univ, Ul Smolina 24a, Ulan Ude 670000, Russia
Sanditov, D. S.
Sangadiev, S. Sh.
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Buryat State Univ, Ul Smolina 24a, Ulan Ude 670000, RussiaBuryat State Univ, Ul Smolina 24a, Ulan Ude 670000, Russia
Sangadiev, S. Sh.
Darmaev, M. V.
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Buryat State Univ, Ul Smolina 24a, Ulan Ude 670000, RussiaBuryat State Univ, Ul Smolina 24a, Ulan Ude 670000, Russia
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Univ Montpellier 2, CNRS, UMR 5221, Lab Charles Coulomb, F-34095 Montpellier, FranceUniv Montpellier 2, CNRS, UMR 5221, Lab Charles Coulomb, F-34095 Montpellier, France
Roldan-Vargas, Sandalo
Berthier, Ludovic
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Univ Montpellier 2, CNRS, UMR 5221, Lab Charles Coulomb, F-34095 Montpellier, FranceUniv Montpellier 2, CNRS, UMR 5221, Lab Charles Coulomb, F-34095 Montpellier, France
Berthier, Ludovic
PROCEEDINGS OF THE 25TH WORKSHOP ON COMPUTER SIMULATION STUDIES IN CONDENSED MATTER PHYSICS,
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