Oxygen carriers for chemical-looping water splitting to hydrogen production: A critical review

被引：37

作者：

Zhao, Longfei ^{[1
]}

Dou, Binlin ^{[1
]}

Zhang, Hua ^{[1
]}

Wang, Zilong ^{[1
]}

机构：

[1] Univ Shanghai Sci & Technol, Sch Energy & Power Engn, Shanghai Key Lab Multiphase Flow & Heat Transfer P, Shanghai 200093, Peoples R China

来源：

CARBON CAPTURE SCIENCE & TECHNOLOGY | 2021年 / 1卷

基金：

中国国家自然科学基金;

关键词：

Hydrogen; Hydrocarbon; Chemical looping; Water splitting; Oxygen carrier; STEAM-IRON PROCESS; ISOTHERMAL REDUCTION KINETICS; PARTIAL OXIDATION; REDOX BEHAVIOR; PURE HYDROGEN; STORING HYDROGEN; MEMBRANE REACTOR; SYNTHESIS GAS; SOLID FUELS; METHANE;

D O I：

10.1016/j.ccst.2021.100006

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

Chemical looping water splitting (CLWS) process using metal oxides or perovskites as oxygen carriers (OCs), is capable of producing pure H 2 in an efficient, simple, and flexible way. The OCs are first reduced by hydrocarbon fuels and then oxidized by steam in a cyclic way. After the condensation of the gaseous mixture of steam and H 2 from the oxidation step, pure H 2 is obtained. In recent years, great efforts for CLWS have been made to improve the redox activity and stability of OCs. In this paper, the development of the OCs for hydrogen production from CLWS were discussed. Effects of supports and additives on the performances of OCs were compared based on redox reactions in CLWS. Fe-based OCs with CeO2, Al2O3, ZrO2, CuO, MoO3, Rh etc. are very attractive for the CLWS process. Issues and challenges for the development of OCs were analyzed.

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页数：10

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