Disentangling boson peaks and Van Hove singularities in a model glass

被引:25
|
作者
Wang, Yinqiao [1 ]
Hong, Liang [1 ,2 ]
Wang, Yujie [1 ]
Schirmacher, Walter [3 ]
Zhang, Jie [1 ,2 ,4 ]
机构
[1] Shanghai Jiao Tong Univ, Sch Phys & Astron, 800 Doug Chuan Rd, Shanghai 200240, Peoples R China
[2] Shanghai Jiao Tong Univ, Inst Nat Sci, Shanghai 200240, Peoples R China
[3] Johannes Gutenberg Univ Mainz, Inst Phys, Staudinger Weg 7, D-55099 Mainz, Germany
[4] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China
关键词
RAMAN-SCATTERING; EXCITATIONS; RELAXATIONS; VIBRATIONS; ANOMALIES; DYNAMICS; SOLIDS;
D O I
10.1103/PhysRevB.98.174207
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Using the example of a two-dimensional macroscopic model glass in which the interparticle forces can be precisely measured, we obtain strong hints for resolving a controversy concerning the origin of the anomalous enhancement of the vibrational spectrum in glasses (boson peak). Whereas many authors attribute this anomaly to the structural disorder, some other authors claim that the short-range order, leading to washed-out Van Hove singularities, would cause the boson-peak anomaly. As in our model system, the disorder-induced and short-range-order-induced features can be completely separated, we are able to discuss the controversy about the boson peak in real glasses in a new light. Our findings suggest that the interpretation of the boson peak in terms of short-range order only, might result from a coincidence of the two phenomena in the materials studied. In general, as we show, the two phenomena both exist, but are two completely separate entities.
引用
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页数:7
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