Decoupling Carrier Concentration and Electron-Phonon Coupling in Oxide Heterostructures Observed with Resonant Inelastic X-Ray Scattering

被引:25
作者
Meyers, D. [1 ,10 ]
Nakatsukasa, Ken [2 ]
Mu, Sai [3 ]
Hao, Lin [2 ]
Yang, Junyi [2 ]
Cao, Yue [1 ,11 ]
Fabbris, G. [4 ]
Miao, Hu [1 ]
Pelliciari, J. [5 ]
McNally, D. [5 ]
Dantz, M. [5 ]
Paris, E. [5 ]
Icarapetrova, E. [4 ]
Choi, Yongseong [4 ]
Haskel, D. [4 ]
Shafer, P. [6 ]
Arenholz, E. [6 ]
Schmitt, Thorsten [5 ]
Berlijn, Tom [7 ,8 ]
Johnston, S. [2 ,9 ]
Liu, Jian [2 ]
Dean, M. P. M. [1 ]
机构
[1] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA
[2] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA
[3] Oak Ridge Natl Lab, Dept Condensed Matter Phys & Mat Sci, Oak Ridge, TN 37830 USA
[4] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA
[5] Paul Scherrer Inst, Photon Sci Div, Swiss Light Source, CH-5232 Villigen, Switzerland
[6] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA
[7] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA
[8] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA
[9] Univ Tennessee, Joint Inst Adv Mat, Knoxville, TN 37996 USA
[10] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA
[11] Argonne Natl Lab, Mat Sci Div, Argonne, IL 60439 USA
基金
瑞士国家科学基金会;
关键词
SUPERCONDUCTIVITY; INTERFACES;
D O I
10.1103/PhysRevLett.121.236802
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report the observation of multiple phonon satellite features in ultrathin superlattices of the form nSrIrO(3)/mSrTiO(3) using resonant inelastic x-ray scattering (RIXS). As the values of n and m vary, the energy loss spectra show a systematic evolution in the relative intensity of the phonon satellites. Using a closed-form solution for the RIXS cross section, we extract the variation in the electron-phonon coupling strength as a function of n and m. Combined with the negligible carrier doping into the SrTiO3 layers, these results indicate that the tuning of the electron-phonon coupling can be effectively decoupled from doping. This work both showcases a feasible method to extract the electron-phonon coupling in superlattices and unveils a potential mute for tuning this coupling, which is often associated with superconductivity in SrTiO3-based systems.
引用
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页数:6
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