Three-dimensional composite hydrogel based on polyamine zirconium oxide, alginate and tannic acid with high performance for Pb(II), Hg(II) and Cr(VI) trapping

被引：20
作者：
Zhang, Yun [1 ]
He, Fu [1 ]
Li, Xiaoli [2 ]
机构：
[1] Lanzhou Univ, Coll Chem & Chem Engn, Lanzhou 730000, Peoples R China
[2] Lanzhou Univ, Coll Resources & Environm Sci, Lanzhou 730000, Peoples R China
来源：
JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS | 2016年 / 65卷
基金：
中国国家自然科学基金;
关键词：
Three-dimensional hydrogels; Polyamine zirconium oxide; Tannic acid; Alginate; Heavy metal trapping; AQUEOUS-SOLUTIONS; HYBRID MATERIAL; METALS REMOVAL; ADSORPTION; LEAD; BIOSORPTION; WATER; NANOPARTICLES; CADMIUM; RESIN;
D O I：
10.1016/j.jtice.2016.05.023
中图分类号：
TQ [化学工业];
学科分类号：
0817 ;
摘要：
In this study, preparation of multifunctional polymer hydrogels (Zr-DETA/TS) was achieved via organic inorganic crosslinking to form three-dimensional network structure for application of Pb2+, Hg2+ and CrO42- extraction. The equilibrium data of Pb2+, Hg2+ and CrO42- were best described by the Langmuir isotherm, and the kinetic data were found to follow the pseudo-second-order kinetic model. It was notable that ionic exchange and complexation were the main adsorption mechanism for Pb2+ and Hg2+ while electrostatic attraction, inner-sphere complex and esterification played an important role in CrO42- adsorption. Thus, Zr-DETA/TS hydrogels could be used as a promising biomaterial for Pb2+, Hg2+ and CrO42- removal from wastewaters. (C) 2016 Taiwan Institute of Chemical Engineers. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码：304 / 311
页数：8
相关论文
共 39 条
[1]   Biosorption of Hg2+, Cd2+, and Zn2+ by Ca-alginate and immobilized wood-rotting fungus Funalia trogii [J].
Arica, MY ;
Bayramoglu, G ;
Yilmaz, M ;
Bektas, S ;
Genç, Ö .
JOURNAL OF HAZARDOUS MATERIALS, 2004, 109 (1-3) :191-199
[2]   Adsorption and removal of As(V) and As(111) using Zr-loaded lysine diacetic acid chelating resin [J].
Balaji, T ;
Yokoyama, T ;
Matsunaga, H .
CHEMOSPHERE, 2005, 59 (08) :1169-1174
[3]   Adsorptive removal of As(V) and As(III) from water by a Zr(IV)-loaded orange waste gel [J].
Biswas, Biplob Kumar ;
Inoue, Jun-ichi ;
Inoue, Katsutoshi ;
Ghimire, Kedar Nath ;
Harada, Hiroyuki ;
Ohto, Keisuke ;
Kawakita, Hidetaka .
JOURNAL OF HAZARDOUS MATERIALS, 2008, 154 (1-3) :1066-1074
[4]   Simultaneous adsorption of lead and cadmium on MnO2-loaded resin [J].
Dong, Lijing ;
Zhu, Zhiliang ;
Ma, Hongmei ;
Qiu, Yanling ;
Zhao, Jianfu .
JOURNAL OF ENVIRONMENTAL SCIENCES, 2010, 22 (02) :225-229
[5]   Removal of aqueous toxic Hg(II) by synthesized TiO2 nanoparticles and TiO2/montmorillonite [J].
Dou, Binlin ;
Dupont, Valerie ;
Pan, Weiguo ;
Chen, Bingbing .
CHEMICAL ENGINEERING JOURNAL, 2011, 166 (02) :631-638
[6]   Biosorption of heavy metals from aqueous solutions by chemically modified orange peel [J].
Feng, Ningchuan ;
Guo, Xueyi ;
Liang, Sha ;
Zhu, Yanshu ;
Liu, Jianping .
JOURNAL OF HAZARDOUS MATERIALS, 2011, 185 (01) :49-54
[7]   Adsorption of Ni2+, Zn2+ and Pb2+ onto dry biomass of Arthrospira (Spirulina) platensis and Chlorella vulgaris. I. Single metal systems [J].
Ferreira, Livia Seno ;
Rodrigues, Mayla Santos ;
Monteiro de Carvalho, Joao Carlos ;
Lodi, Alessandra ;
Finocchio, Elisabetta ;
Perego, Patrizia ;
Converti, Attilio .
CHEMICAL ENGINEERING JOURNAL, 2011, 173 (02) :326-333
[8]   LEAD TOXICITY - CURRENT CONCERNS [J].
GOYER, RA .
ENVIRONMENTAL HEALTH PERSPECTIVES, 1993, 100 :177-187
[9]   Adsorption of chromium (VI) by ethylenediamine-modified cross-linked magnetic chitosan resin: Isotherms, kinetics and thermodynamics [J].
Hu, Xin-jiang ;
Wang, Jing-song ;
Liu, Yun-guo ;
Li, Xin ;
Zeng, Guang-ming ;
Bao, Zheng-lei ;
Zeng, Xiao-xia ;
Chen, An-wei ;
Long, Fei .
JOURNAL OF HAZARDOUS MATERIALS, 2011, 185 (01) :306-314
[10]   Removal of arsenate by cetyltrimethylammonium bromide modified magnetic nanoparticles [J].
Jin, Yinjia ;
Liu, Fei ;
Tong, Meiping ;
Hou, Yanglong .
JOURNAL OF HAZARDOUS MATERIALS, 2012, 227 :461-468
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