Organic and perovskite solar modules innovated by adhesive top electrode and depth-resolved laser patterning

被引：69

作者：

Spyropoulos, George D. ^{[1
]}

Quiroz, Cesar Omar Ramirez ^{[2
]}

Salvador, Michael ^{[2
,3
]}

Hou, Yi ^{[2
,4
]}

Gasparini, Nicola ^{[2
]}

Schweizer, Peter ^{[5
]}

Adams, Jens ^{[1
]}

Kubis, Peter ^{[1
,4
]}

Li, Ning ^{[2
]}

Spiecker, Erdmann ^{[5
]}

Ameri, Tayebeh ^{[2
]}

Egelhaaf, Hans-Joachim ^{[1
]}

Brabec, Christoph J. ^{[1
,2
]}

机构：

[1] ZAE Bayern Solar Factory Future, Energy Campus Nurnberg,Furthersttrasse 250, D-90429 Nurnberg, Germany

[2] Univ Erlangen Nurnberg, i MEET, Martensstr 7, D-91058 Erlangen, Germany

[3] Inst Super Tecn, Inst Telecomunicacoes, Ave Rovisco Pais, P-1049001 Lisbon, Portugal

[4] Erlangen Grad Sch Adv Opt Technol SAOT, Paul Gordan Str 6, D-91052 Erlangen, Germany

[5] Univ Erlangen Nurnberg, Ctr Nanoanal & Electron Microscopy CENEM, Cauerstr 6, D-91058 Erlangen, Germany

来源：

ENERGY & ENVIRONMENTAL SCIENCE | 2016年 / 9卷 / 07期

关键词：

PHOTOVOLTAIC DEVICES; LAMINATION PROCESS; CELLS; FABRICATION; HYSTERESIS; LAYER; AIR;

D O I：

10.1039/c6ee01555g

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

We demonstrate an innovative solution-processing fabrication route for organic and perovskite solar modules via depth-selective laser patterning of an adhesive top electrode. This yields unprecedented power conversion efficiencies of up to 5.3% and 9.8%, respectively. We employ a PEDOT:PSS-Ag nanowire composite electrode and depth-resolved post-patterning through beforehand laminated devices using ultra-fast laser scribing. This process affords low-loss interconnects of consecutive solar cells while overcoming typical alignment constraints. Our strategy informs a highly simplified and universal approach for solar module fabrication that could be extended to other thin-film photovoltaic technologies.

引用

页码：2302 / 2313

页数：12

共 52 条

[41] Origin and elimination of photocurrent hysteresis by fullerene passivation in CH3NH3PbI3 planar heterojunction solar cells [J].

Shao, Yuchuan ;

Xiao, Zhengguo ;

Bi, Cheng ;

Yuan, Yongbo ;

Huang, Jinsong .

NATURE COMMUNICATIONS, 2014, 5

[42] Viscous Conductive Glue Layer in Semitransparent Polymer-Based Solar Cells Fabricated by a Lamination Process [J].

Shimada, Chieko ;

Shiratori, Seimei .

ACS APPLIED MATERIALS & INTERFACES, 2013, 5 (21) :11087-11092

[43] Roll-to-roll fabrication of polymer solar cells [J].

Sondergaard, Roar ;

Hosel, Markus ;

Angmo, Dechan ;

Larsen-Olsen, Thue T. ;

Krebs, Frederik C. .

MATERIALS TODAY, 2012, 15 (1-2) :36-49

[44] Flexible organic tandem solar modules with 6% efficiency: combining roll-to-roll compatible processing with high geometric fill factors [J].

Spyropoulos, G. D. ;

Kubis, P. ;

Li, N. ;

Baran, D. ;

Lucera, L. ;

Salvador, M. ;

Ameri, T. ;

Voigt, M. M. ;

Krebs, F. C. ;

Brabec, C. J. .

ENERGY & ENVIRONMENTAL SCIENCE, 2014, 7 (10) :3284-3290

[45] Laminated fabric as top electrode for organic photovoltaics [J].

Steim, R. ;

Chabrecek, P. ;

Sonderegger, U. ;

Kindle-Hasse, B. ;

Siefert, W. ;

Kroyer, T. ;

Reinecke, P. ;

Lanz, T. ;

Geiger, T. ;

Hany, R. ;

Nueesch, F. .

APPLIED PHYSICS LETTERS, 2015, 106 (19)

[46] Degradation of a Thin Ag Layer Induced by Poly(3,4ethylenedioxythiophene):Polystyrene Sulfonate in a Transmission Electron Microscopy Specimen of an Inverted Polymer Solar Cell [J].

Suh, Youngjoon ;

Lu, Ning ;

Lee, Sang H. ;

Chung, Won-Suk ;

Kim, Kyungkon ;

Kim, BongSoo ;

Ko, Min Jae ;

Kim, Moon J. .

ACS APPLIED MATERIALS & INTERFACES, 2012, 4 (10) :5118-5124

[47]

Tada A, 2011, NAT MATER, V10, P450, DOI [10.1038/nmat3026, 10.1038/NMAT3026]

[48] Sticky Interconnect for Solution-Processed Tandem Solar Cells [J].

Tung, Vincent C. ;

Kim, Jaemyung ;

Cote, Laura J. ;

Huang, Jiaxing .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (24) :9262-9265

[49] Efficient and non-hysteresis CH3NH3PbI3/PCBM planar heterojunction solar cells [J].

Xiong, Jian ;

Yang, Bingchu ;

Wu, Runsheng ;

Cao, Chenghao ;

Huang, Yulan ;

Liu, Chengbin ;

Hu, Zhikun ;

Huang, Han ;

Gao, Yongli ;

Yang, Junliang .

ORGANIC ELECTRONICS, 2015, 24 :106-112

[50] Achieving high efficiency laminated polymer solar cell with interfacial modified metallic electrode and pressure induced crystallization [J].

Yuan, Yongbo ;

Bi, Yu ;

Huang, Jinsong .

APPLIED PHYSICS LETTERS, 2011, 98 (06)

← 1 2 3 4 5 6 →