ABOVE THRESHOLD IONIZATION OF POLAR NaK MOLECULES DRIVEN BY FEW-CYCLE LASER PULSE

被引:10
作者
Yu, Jie [1 ]
Shu, Chuan-Cun [1 ]
Hu, Wen-Hui [1 ]
Cong, Shu-Lin [1 ]
机构
[1] Dalian Univ Technol, Sch Phys & Optoelect Technol, Dalian 116024, Peoples R China
基金
中国国家自然科学基金;
关键词
Above-threshold ionization; carrier-envelope phase; molecular orientation; MULTIPHOTON IONIZATION; ABSOLUTE-PHASE; PHOTOIONIZATION; FEMTOSECOND; ASYMMETRY;
D O I
10.1142/S0219633610006018
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We investigate theoretically the above-threshold ionization (ATI) of the polar NaK molecule exposed in few-cycle laser field by numerically solving the time-dependent Schrodinger equation including the vibrational and rotational degrees of freedom. The left and right ATI spectra are calculated by integrating the ionization continuum wave function over the left and the right half spheres along the laser polarization. We find that the left and right ATI spectra are asymmetric, and this asymmetry depends strongly on the molecular orientation and the carrier-envelope phase (CEP) of the laser pulse. Moreover, we also perform the calculation for different initially rotational states to study the effect of rotational temperature on the ATI dynamics.
引用
收藏
页码:785 / 795
页数:11
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