A critical review of the influence of groundwater level fluctuations and temperature on LNAPL contaminations in the context of climate change

被引:63
作者
Cavelan, Amelie [1 ]
Golfier, Fabrice [2 ]
Colombano, Stefan [3 ]
Davarzani, Hossein [3 ]
Deparis, Jacques [3 ]
Faure, Pierre [1 ]
机构
[1] Univ Lorraine, CNRS, LIEC, F-54000 Nancy, France
[2] Univ Lorraine, CNRS, GeoRessources, F-54000 Nancy, France
[3] BRGM French Geol Survey, F-45100 Orleans, France
关键词
Light non-aqueous phase liquids; Groundwater; Dissolution; Biodegradation; Volatilization; NONAQUEOUS-PHASE LIQUID; SATURATED SUBSURFACE SYSTEMS; WATER-TABLE FLUCTUATIONS; ZONE DEPLETION PROCESSES; HISTORIC FLUID LEVELS; MASS-TRANSFER; ORGANIC-COMPOUNDS; ANALYTICAL-MODEL; MICROBIAL COMMUNITY; AQUEOUS SOLUBILITY;
D O I
10.1016/j.scitotenv.2021.150412
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The intergovernmental panel on climate change (IPCC) predicts significant changes in precipitation patterns, an increase in temperature, and groundwater level variations by 2100. These changes are expected to alter light non-aqueous phase liquid (LNAPL) impacts since groundwater level fluctuations and temperature are known to influence both the mobility and release of LNAPL compounds to air and groundwater. Knowledge of these po-tential effects is currently dispersed in the literature, hindering a clear vision of the processes at play. This review aims to synthesize and discuss the possible effects of the increase in temperature and groundwater level fluctu-ations on the behavior of LNAPL and its components in a climate change context. In summary, a higher amplitude of groundwater table variations and higher temperatures will probably increase biodegradation processes, the LNAPL mobility, and spreading across the smear zone, favoring the release of LNAPL compounds to the atmo-sphere and groundwater but decreasing the LNAPL mass and its longevity. Outcomes will, nevertheless, vary greatly across arid, cold, or humid coastal environments, where different effects of climate change are expected. The effects of the climate change factors linked to soil heterogeneities, local conditions, and weathering processes will govern LNAPL behavior and need to be further clarified. (c) 2021 Elsevier B.V. All rights reserved.
引用
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页数:15
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