Combination of MOFs and Zeolites for Mixed-Matrix Membranes

被引：226
|
作者：
Zornoza, Beatriz [1 ,2 ]
Seoane, Beatriz [1 ,2 ]
Zamaro, Juan M. [3 ]
Tellez, Carlos [1 ,2 ]
Coronas, Joaquin [1 ,2 ]
机构：
[1] Univ Zaragoza, Chem & Environm Engn Dept, Zaragoza 50018, Spain
[2] Univ Zaragoza, Inst Nanociencia Aragon, Zaragoza 50018, Spain
[3] Consejo Nacl Invest Cient & Tecn, FIQ, UNL, Inst Invest Catalisis & Petroquim INCAPE, RA-3000 Santa Fe, Argentina
来源：
CHEMPHYSCHEM | 2011年 / 12卷 / 15期
关键词：
gas separation; membranes; metal-organic frameworks; organic-inorganic hybrid composites; zeolites; GAS-PERMEABILITY PROPERTIES; COMPOSITE MEMBRANES; POLYSULFONE; SEPARATION; DESIGN;
D O I：
10.1002/cphc.201100583
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Mixed-matrix membranes (MMMs) were prepared by combinations of two different kinds of porous fillers [metal-organic frameworks (MOFs) HKUST-1 and ZIF-8, and zeolite silicalite-1] and polysulfone. In the search for filler synergy, the MMMs were applied to the separation of CO2/N-2, CO2/CH4, O-2/N-2, and H-2/CH4 mixtures and we found important selectivity improvements with the HKUST-1-silicalite-1 system (CO2/CH4 and CO2/N-2 separation factors of 22.4 and 38.0 with CO2 permeabilities of 8.9 and 8.4 Barrer, respectively).
引用
收藏
页码：2781 / 2785
页数：5
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