TiO2;
HF treatment;
water splitting;
photocatalysis;
photoelectrochemistry;
D O I:
10.1163/156856708784795518
中图分类号:
O6 [化学];
学科分类号:
0703 ;
摘要:
The effects of HF treatment on the activity of TiO2 thin films for the photocatalytic water splitting reaction have been investigated. TiO2 thin films treated with HF solution (HF-TiO2) were found to exhibit a remarkable enhancement of the photocatalytic activity for H-2 evolution from a methanol aqueous solution, as well as efficient photoelectrochemical performance under UV light irradiation as compared with the untreated TiO2. Moreover, Pt-loaded HF-TiO2 thin films were found to act as efficient and stable photocatalysts for the decomposition of water under UV light irradiation. The mechanistic insights obtained in the present study will be useful in the design of highly efficient photocatalysts for the decomposition of water.
机构:
Chinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R ChinaChinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R China
Yu, R. S.
Qin, X. B.
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机构:
Chinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R ChinaChinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R China
Qin, X. B.
Wang, Q. Z.
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Chinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R ChinaChinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R China
Wang, Q. Z.
Zhang, P.
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Chinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R ChinaChinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R China
Zhang, P.
Wang, B. Y.
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Chinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R ChinaChinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R China
Wang, B. Y.
Wei, L.
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Chinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R ChinaChinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R China
Wei, L.
Hao, W. C.
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机构:
Beihang Univ, Ctr Mat Phys & Chem, Beijing 100083, Peoples R ChinaChinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R China
Hao, W. C.
Wang, T. M.
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机构:
Beihang Univ, Ctr Mat Phys & Chem, Beijing 100083, Peoples R ChinaChinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R China