Atmospheric Mercury Outflow from China and Interprovincial Trade

被引:18
作者
Chen, Long [1 ,2 ]
Liang, Sai [3 ]
Zhang, Yanxu [4 ]
Liu, Maodian [5 ]
Meng, Jing [6 ]
Zhang, Haoran [5 ]
Tang, Xi [1 ,2 ]
Li, Yumeng [3 ]
Tong, Yindong [7 ]
Zhang, Wei [8 ]
Wang, Xuejun [5 ]
Shu, Jiong [1 ,2 ]
机构
[1] East China Normal Univ, Key Lab Geog Informat Sci, Minist Educ, Shanghai 200241, Peoples R China
[2] East China Normal Univ, Sch Geog Sci, Shanghai 200241, Peoples R China
[3] Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China
[4] Nanjing Univ, Sch Atmospher Sci, Nanjing 210023, Jiangsu, Peoples R China
[5] Peking Univ, Coll Urban & Environm Sci, Minist Educ, Lab Earth Surface Proc, Beijing 100871, Peoples R China
[6] Univ Cambridge, Dept Polit & Int Studies, Cambridge CB3 9DT, England
[7] Tianjin Univ, Sch Environm Sci & Engn, Tianjin 300072, Peoples R China
[8] Renmin Univ China, Sch Environm & Nat Resources, Beijing 100872, Peoples R China
基金
中国国家自然科学基金; 中国博士后科学基金;
关键词
METHYLMERCURY EXPOSURE; INTERNATIONAL-TRADE; DEPOSITION; EMISSIONS; FISH; TRANSPORT; MODEL; CO2;
D O I
10.1021/acs.est.8b03951
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Mercury (Hg) is characterized by its ability to migrate between continents and its adverse effects on human health, arousing great concern around the world. The transboundary transport of large anthropogenic Hg emissions from China has attracted particular attention, especially from neighboring countries. Here, we combine an atmospheric transport model, a mass budget analysis, and a multiregional input-output model to simulate the atmospheric Hg outflow from China and investigate the impacts of Chinese interprovincial trade on the outflow. The results show outflows of 423.0 Mg of anthropogenic Hg, consisting of 65.9% of the total Chinese anthropogenic emissions, from China in 2010. Chinese interprovincial trade promotes the transfer of atmospheric outflow from the eastern terrestrial boundary (-6.4 Mg year(-1)) to the western terrestrial boundary (+4.5 Mg year(-1)) and a net decrease in the atmospheric outflow for the whole boundary, reducing the chance of risks to foreign countries derived from transboundary Hg pollution from China. These impacts of interprovincial trade will be amplified due to the expected strengthened interprovincial trade in the future. The synergistic promotional effects of interprovincial trade versus Hg controls should be considered to reduce the transboundary Hg pollution from China.
引用
收藏
页码:13792 / 13800
页数:9
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