Tailored synthesis of SnO2@graphene nanocomposites with enhanced photocatalytic response

被引:32
作者
Chen, Haitao [1 ,2 ]
Pu, Xuemei [1 ]
Gu, Ming [1 ]
Zhu, Jun [1 ]
Cheng, Liwen [1 ]
机构
[1] Yangzhou Univ, Coll Phys Sci & Technol, Yangzhou 225002, Jiangsu, Peoples R China
[2] Nanjing Univ, Natl Lab Solid State Microstruct, Lab Modern Acoust MOE, Nanjing 210093, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
Nanocomposite; Photocatalytic property; Charge separation; TIN-OXIDE; PERFORMANCE; SNO2; NANOSTRUCTURES; GRAPHENE; SNO2/GRAPHENE; OXYGEN; ZNO;
D O I
10.1016/j.ceramint.2016.08.095
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Hierarchical SnO2@graphene nanocomposites were synthesized by impregnating different weight percentages of Sn2+ with graphene oxide nanosheets using a simple hydrothermal method. The precursor ratio of Sn2+ to graphene oxide plays a decisive role in tailoring the phase structure and composition, which thereby influences the photocatalytic performance to degrade the organic contaminants. The SnO2@graphene nanocomposites exhibited greatly enhanced abilities for photocatalytic degradation of MO dye compare with the pure SnO2. It is believed that the tight heterojunction structure and efficient charge separation play important roles in facilitating interfacial electron transfer and reducing self-radiative recombination of charges, which accordingly enhance the photocatalytic performance. (C) 2016 Elsevier Ltd and Techna Group S.r.l. All rights reserved.
引用
收藏
页码:17717 / 17722
页数:6
相关论文
共 25 条
  • [1] Solid-state synthesis of SnO2-graphene nanocomposite for photocatalysis and formaldehyde gas sensing
    Cao, Yali
    Li, Yizhao
    Jia, Dianzeng
    Xie, Jing
    [J]. RSC ADVANCES, 2014, 4 (86) : 46179 - 46186
  • [2] Interaction of oxygen and carbon monoxide with CsAu surfaces
    Carley, AF
    Roberts, MW
    Santra, AK
    [J]. JOURNAL OF PHYSICAL CHEMISTRY B, 1997, 101 (48): : 9978 - 9983
  • [3] Fabrication of SnO2@SnS2 heterostructure with enhanced visible light photocatalytic activity
    Chen, Haitao
    Gu, Ming
    Pu, Xuemei
    Zhu, Jun
    Cheng, Liwen
    [J]. MATERIALS RESEARCH EXPRESS, 2016, 3 (06):
  • [4] Controllable construction of ordered porous SnO2 nanostructures and their application in photocatalysis
    Chen, Haitao
    Zhang, Dan
    Zhou, Xuming
    Zhu, Jun
    Chen, Xiaobing
    Zeng, Xianghua
    [J]. MATERIALS LETTERS, 2014, 116 : 127 - 130
  • [5] Enhancement of Field Emission and Photoluminescence Properties of Graphene-SnO2 Composite Nanostructures
    Ding, Jijun
    Yan, Xingbin
    Li, Jun
    Shen, Baoshou
    Yang, Juan
    Chen, Jiangtao
    Xue, Qunji
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2011, 3 (11) : 4299 - 4305
  • [6] One-step synthesis of graphene/SnO2 nanocomposites and its application in electrochemical supercapacitors
    Li, Fenghua
    Song, Jiangfeng
    Yang, Huafeng
    Gan, Shiyu
    Zhang, Qixian
    Han, Dongxue
    Ivaska, Ari
    Niu, Li
    [J]. NANOTECHNOLOGY, 2009, 20 (45)
  • [7] Preparation and characterization of tin oxide, SnO2 nanoparticles decorated graphene
    Lim, H. N.
    Nurzulaikha, R.
    Harrison, I.
    Lim, S. S.
    Tan, W. T.
    Yeo, M. C.
    Yarmo, M. A.
    Huang, N. M.
    [J]. CERAMICS INTERNATIONAL, 2012, 38 (05) : 4209 - 4216
  • [8] Reduced Graphene Oxide-Hierarchical ZnO Hollow Sphere Composites with Enhanced Photocurrent and Photocatalytic Activity
    Luo, Qiu-Ping
    Yu, Xiao-Yun
    Lei, Bing-Xin
    Chen, Hong-Yan
    Kuang, Dai-Bin
    Su, Cheng-Yong
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2012, 116 (14) : 8111 - 8117
  • [9] Synthesis and electrocatalytic performance of nitrogen-doped macroporous carbons
    Meng, Xin
    Cui, Huijuan
    Dong, Jianhui
    Zheng, Jianfeng
    Zhu, Yanyan
    Wang, Zhijian
    Zhang, Jian
    Jia, Suping
    Zhao, Jianghong
    Zhu, Zhenping
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2013, 1 (33) : 9469 - 9476
  • [10] Hydrothermal synthesis of Ti oxide nanostructures and TiO2:SnO2 heterostructures applied to the photodegradation of rhodamine B
    Mourao, Henrique A. J. L.
    Avansi Junior, Waldir
    Ribeiro, Caue
    [J]. MATERIALS CHEMISTRY AND PHYSICS, 2012, 135 (2-3) : 524 - 532