Magneto-optical study of the spin-polarized electronic states in multiferroic TbMnO3

被引:23
作者
Bastjan, M. [1 ]
Singer, S. G. [1 ]
Neuber, G. [1 ]
Eller, S. [1 ]
Aliouane, N. [2 ]
Argyriou, D. N. [2 ]
Cooper, S. L. [3 ,4 ]
Rubhausen, M. [1 ]
机构
[1] Univ Hamburg, Inst Angew Phys, D-20355 Hamburg, Germany
[2] Hahn Meitner Inst Berlin GmbH, D-14109 Berlin, Germany
[3] Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA
[4] Univ Illinois, Dept Phys, Urbana, IL 61801 USA
关键词
D O I
10.1103/PhysRevB.77.193105
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The magnetic and electronic properties of multiferroic TbMnO3 in the paramagnetic, antiferromagnetic, sinusoidal, and spiral-spin phases were studied by spectral generalized magneto-optical ellipsometry. The measurements show a strong anisotropy of the dielectric tensor. A redistribution of spectral weight was observed in the diagonal components of the dielectric tensor for the temperature range from 110 to T-N = 46 K. In the off-diagonal elements, spectral generalized magneto-optical ellipsometry shows sensitivity to the antiferromagnetic and ferroelectric phase transitions at T-N = 46 K and T-F = 29 K, respectively, and a persistent signal up to 6T(N).
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页数:3
相关论文
共 18 条
[1]   Field-induced linear magnetoelastic coupling in multiferroic TbMnO3 -: art. no. 020102 [J].
Aliouane, N ;
Argyriou, DN ;
Strempfer, J ;
Zegkinoglou, I ;
Landsgesell, S ;
Zimmermann, MV .
PHYSICAL REVIEW B, 2006, 73 (02)
[2]   FARADAY EFFECT IN SOLIDS [J].
BENNETT, HS ;
STERN, EA .
PHYSICAL REVIEW, 1965, 137 (2A) :A448-+
[3]   Generalized magneto-optical ellipsometry [J].
Berger, A ;
Pufall, MR .
APPLIED PHYSICS LETTERS, 1997, 71 (07) :965-967
[4]   A THERMODYNAMIC THEORY OF WEAK FERROMAGNETISM OF ANTIFERROMAGNETICS [J].
DZYALOSHINSKY, I .
JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS, 1958, 4 (04) :241-255
[5]   Revival of the magnetoelectric effect [J].
Fiebig, M .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2005, 38 (08) :R123-R152
[6]   Magnetic inversion symmetry breaking and ferroelectricity in TbMnO3 -: art. no. 087206 [J].
Kenzelmann, M ;
Harris, AB ;
Jonas, S ;
Broholm, C ;
Schefer, J ;
Kim, SB ;
Zhang, CL ;
Cheong, SW ;
Vajk, OP ;
Lynn, JW .
PHYSICAL REVIEW LETTERS, 2005, 95 (08)
[7]   Effect of orbital rotation and mixing on the optical properties of orthorhombic RMnO3 (R=La, Pr, Nd, Gd, and Tb) [J].
Kim, M. W. ;
Moon, S. J. ;
Jung, J. H. ;
Yu, Jaejun ;
Parashar, Sachin ;
Murugavel, P. ;
Lee, J. H. ;
Noh, T. W. .
PHYSICAL REVIEW LETTERS, 2006, 96 (24)
[8]   Origin of the 2 eV peak in optical absorption spectra of LaMnO3:: an explanation based on the orbitally degenerate Hubbard model -: art. no. 156 [J].
Kim, MW ;
Murugavel, P ;
Parashar, S ;
Lee, JS ;
Noh, TW .
NEW JOURNAL OF PHYSICS, 2004, 6 :1-12
[9]  
KIMURA T, 2003, NATURE, V55, P426
[10]   Spin-controlled mott-hubbard bands in LaMnO3 probed by optical ellipsometry -: art. no. 147204 [J].
Kovaleva, NN ;
Boris, AV ;
Bernhard, C ;
Kulakov, A ;
Pimenov, A ;
Balbashov, AM ;
Khaliullin, G ;
Keimer, B .
PHYSICAL REVIEW LETTERS, 2004, 93 (14) :147204-1