Synthesis and Characterization of Solution-Processable Ladderized n-Type Naphthalene Bisimide Copolymers for OFET Applications

被引：100

作者：

Durban, Matthew M. ^{[2
]}

Kazarinoff, Peter D. ^{[1
]}

Segawa, Yukari ^{[1
,3
]}

Luscombe, Christine K. ^{[1
]}

机构：

[1] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA

[2] Univ Washington, Dept Chem, Seattle, WA 98195 USA

[3] Tokyo Inst Technol, Grad Sch Engn, Dept Organ & Polymer Mat, Meguro Ku, Tokyo 1528552, Japan

来源：

MACROMOLECULES | 2011年 / 44卷 / 12期

基金：

美国国家科学基金会;

关键词：

THIN-FILM TRANSISTORS; INTRAMOLECULAR CHARGE-TRANSFER; FIELD-EFFECT TRANSISTORS; HIGH-ELECTRON-MOBILITY; DIIMIDE SEMICONDUCTORS; ORGANIC SEMICONDUCTORS; HIGH-PERFORMANCE; PI-CONJUGATION; POLYMERS; PLANAR;

D O I：

10.1021/ma2004822

中图分类号：

O63 [高分子化学（高聚物）];

学科分类号：

070305 ; 080501 ; 081704 ;

摘要：

Solution-processable n-type ladder-based polymers are highly desirable due to their potential capability to form strong. pi-pi interactions. A series of 5 highly soluble naphthalene diimide (NDI) polymers are presented, differing in the degree to which they are able to form imine-bridged ladder polymer structures. Average electron mobilities as high as 0.0026 cm(2) V-1 s(-1), which show an electron-mobility improvement of 4 orders of magnitude following ladderization, and on/off current ratios on the order of 10(4) are reported for the novel material PNDI-2BocL, an alkyl-substituted poly(benzoquinolinophenanthrolinedione). The structure property relationship of the aforementioned series of copolymers is presented and discussed as it pertains to organic field-effect transistor (OFET) performance.

引用

页码：4721 / 4728

页数：8

共 50 条

[31] Self-condensation-type direct arylation synthesis of naphthalene bisimide-bithiophene alternating copolymers [J].

Nakabayashi, Kazuhiro ;

Fukuzawa, Haruka ;

Yamada, Masaya ;

Mori, Hideharu .

MICROSYSTEM TECHNOLOGIES-MICRO-AND NANOSYSTEMS-INFORMATION STORAGE AND PROCESSING SYSTEMS, 2017, 23 (08) :3817-3823

[32] Self-condensation-type direct arylation synthesis of naphthalene bisimide-bithiophene alternating copolymers [J].

Kazuhiro Nakabayashi ;

Haruka Fukuzawa ;

Masaya Yamada ;

Hideharu Mori .

Microsystem Technologies, 2017, 23 :3817-3823

[33] Synthesis and characterization of benzo[b]thieno[2,3-d]thiophene (BTT) derivatives as solution-processable organic semiconductors for organic field-effect transistors [J].

Lee, Yongchul ;

Ryu, Soomin ;

Choi, Eunjin ;

Ho, Dongil ;

Earmme, Taeshik ;

Kim, Choongik ;

Seo, SungYong .

SYNTHETIC METALS, 2021, 282 (282)

[34] Solution-processed core-extended naphthalene diimides toward organic n-type and ambipolar semiconductors [J].

Luo, Hewei ;

Cai, Zhengxu ;

Tan, Luxi ;

Guo, Yunlong ;

Yang, Ge ;

Liu, Zitong ;

Zhang, Guanxin ;

Zhang, Deqing ;

Xu, Wei ;

Liu, Yunqi .

JOURNAL OF MATERIALS CHEMISTRY C, 2013, 1 (15) :2688-2695

[35] Solution-Processable, Transparent Polyimide for High-Performance High-k Nanocomposite: Synthesis, Characterization, and Dielectric Applications in Transistors [J].

Yu, Yang-Yen ;

Chiu, Chi-Ting ;

Chueh, Chu-Chen .

ASIAN JOURNAL OF ORGANIC CHEMISTRY, 2018, 7 (11) :2263-2270

[36] Solution-Processable Low-Voltage and Flexible Floating-Gate Memories Based on an n-Type Polymer Semiconductor and High-k Polymer Gate Dielectrics [J].

Li, Jinhua ;

Yan, Feng .

ACS APPLIED MATERIALS & INTERFACES, 2014, 6 (15) :12815-12820

[37] Core-Fluorinated Naphthalene Diimides: Synthesis, Characterization, and Application in n-Type Organic Field-Effect Transistors [J].

yuan, Zhongyi ;

Ma, Yingjie ;

Gessner, Thomas ;

Li, Mengmeng ;

Chen, Long ;

Eustachi, Michael ;

Weitz, R. Thomas ;

Li, Chen ;

Muellen, Klaus .

ORGANIC LETTERS, 2016, 18 (03) :456-459

[38] Solution-Processable Star-Shaped Conjugated Molecules with Multiple p-n Branches: Synthesis and Photovoltaic Properties [J].

Fan, Xiaochun ;

Wang, Fang ;

Li, Xiangchun ;

Chen, Yao ;

Lai, Wenyong ;

Huang, Wei .

CHINESE JOURNAL OF ORGANIC CHEMISTRY, 2014, 34 (10) :2027-2034

[39] Air-Stable n-Type Organic Field-Effect Transistors Based on Solution-Processable, Electronegative Oligomers Containing Dicyanomethylene-Substituted Cyclopenta[b]thiophene [J].

Ie, Yutaka ;

Nishida, Kazufumi ;

Karakawa, Makoto ;

Tada, Hirokazu ;

Asano, Atsushi ;

Saeki, Akinori ;

Seki, Shu ;

Aso, Yoshio .

CHEMISTRY-A EUROPEAN JOURNAL, 2011, 17 (17) :4750-4758

[40] Solution-processable donor-π-acceptor type thieno[3,2-b]thiophene derivatives; synthesis, photophysical properties and applications [J].

Isci, Recep ;

Wan, Li ;

Topal, Sebahat ;

Gunturkun, Dilara ;

Campbell, Alasdair James ;

Ozturk, Turan .

JOURNAL OF MATERIALS CHEMISTRY C, 2022, 10 (29) :10719-10727

← 1 2 3 4 5 →