Modulating photoelectronic performance of metal-organic frameworks for premium photocatalysis

被引：142

作者：

Zhang, Tiexin ^{[1
]}

Jin, Yunhe ^{[2
]}

Shi, Yusheng ^{[1
]}

Li, Mochen ^{[1
]}

Li, Jianing ^{[1
]}

Duan, Chunying ^{[1
,2
,3
]}

机构：

[1] Dalian Univ Technol, State Key Lab Fine Chem, Dalian 116024, Peoples R China

[2] Dalian Univ Technol, Zhang Dayu Sch Chem, Dalian 116024, Peoples R China

[3] Collaborat Innovat Ctr Chem Sci & Engn, Tianjin 300071, Peoples R China

来源：

COORDINATION CHEMISTRY REVIEWS | 2019年 / 380卷

基金：

中国国家自然科学基金;

关键词：

FE-BASED MOFS; ENERGY-TRANSFER; COORDINATION POLYMERS; HYDROGEN-PRODUCTION; CO2; REDUCTION; ARTIFICIAL PHOTOSYNTHESIS; PHOTOREDOX CATALYSIS; CHARGE SEPARATION; ARYL HALIDES; BAND-GAP;

D O I：

10.1016/j.ccr.2018.10.001

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

As inorganic-organic hybrid materials, metal-organic frameworks (MOFs) exhibit the combined advantages of inorganic semiconductor-type photocatalysts and organic/organometallic molecular photocatalysts in the field of solar energy conversion. The excited states, charge separations, and charge mobilities of MOFs remarkably influence the results of MOF-based photocatalytic systems, which reflect varying degrees of characteristics of inorganic semiconductors and organic/organometallic dyes. In this review, we aim to examine how the aforementioned photoelectronic performances affect each step of the photocatalytic processes based on the recent advances of energy catalysis and organic transformations by using MOFs, and attempt to find new clues for modulating the photoelectronic properties of MOF-based catalytic systems to achieve premium photocatalytic efficiencies and selectivities. (C) 2018 Elsevier B.V. All rights reserved.

引用

页码：201 / 229

页数：29

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