Artificial Photosynthesis: From Molecular Catalysts for Light-driven Water Splitting to Photoelectrochemical Cells

被引：253

作者：

Andreiadis, Eugen S. ^{[1
]}

Chavarot-Kerlidou, Murielle ^{[1
]}

Fontecave, Marc ^{[1
,2
]}

Artero, Vincent ^{[1
]}

机构：

[1] Univ Grenoble 1, CNRS, CEA, Lab Chim & Biol Met,DSV iRTSV K, Grenoble, France

[2] Coll France, F-75231 Paris, France

来源：

PHOTOCHEMISTRY AND PHOTOBIOLOGY | 2011年 / 87卷 / 05期

关键词：

ACTIVE-SITE MODEL; PHOTOINDUCED HYDROGEN EVOLUTION; OXYGEN-EVOLVING COMPLEX; VISIBLE-LIGHT; IRON HYDROGENASE; ELECTRON-TRANSFER; POLYPYRIDINE COMPLEXES; HOMOGENEOUS CATALYSIS; FUNCTIONAL MODELS; ENERGY-CONVERSION;

D O I：

10.1111/j.1751-1097.2011.00966.x

中图分类号：

Q5 [生物化学]; Q7 [分子生物学];

学科分类号：

071010 ; 081704 ;

摘要：

Photosynthesis has been for many years a fascinating source of inspiration for the development of model systems able to achieve efficient light-to-chemical energetic transduction. This field of research, called "artificial photosynthesis," is currently the subject of intense interest, driven by the aim of converting solar energy into the carbon-free fuel hydrogen through the light-driven water splitting. In this review, we highlight the recent achievements on light-driven water oxidation and hydrogen production by molecular catalysts and we shed light on the perspectives in terms of implementation into water splitting technological devices.

引用

页码：946 / 964

页数：19

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