Schottky-like anomaly in the low-temperature specific heat of single-crystal NdMnO3

被引:19
作者
Cheng, JG [1 ]
Sui, Y [1 ]
Qian, ZN [1 ]
Liu, ZG [1 ]
Miao, JP [1 ]
Huang, XQ [1 ]
Lu, Z [1 ]
Li, Y [1 ]
Wang, XJ [1 ]
Su, WH [1 ]
机构
[1] Harbin Inst Technol, CCMST, Dept Appl Phys, Harbin 150001, Peoples R China
基金
中国国家自然科学基金;
关键词
magnetically ordered materials; heat capacity;
D O I
10.1016/j.ssc.2005.02.009
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The specific heat of single-crystal NdMnO3 was investigated from 2 to 20 K under different magnetic fields up to 8 T. All the specific heat data show a Schottky-like anomaly, which becomes more indistinctive as increasing magnetic field. The experiment data were successfully fitted by taking into account factors such as crystal-field splitting, the two-level Schottky anomaly, the lattice vibration, and type-A anti ferromagnetic (A-AF) spin waves. It was found that the splitting of the ground state doublet of Nd3+ ion increases linearly with magnetic field. The above phenomena can be interpreted in terms of the model of unchanged effective molecular field at Nd3+ site caused by the ferromagnetic component of A-AF structure of Mn spins. This ferromagnetic component is likely caused by the GdFeO3-type octahedron rotation. In addition, it was also found that the magnetic field increases the spin-wave stiffness coefficient, but reduces the Debye temperature. (c) 2005 Elsevier Ltd. All rights reserved.
引用
收藏
页码:381 / 384
页数:4
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