Field-free orientation of molecules with small permanent dipole moments by using a train of half-cycle pulses

被引:0
作者
Chi, FP [1 ]
Chen, JG [1 ]
Chen, G [1 ]
Yang, YJ [1 ]
Zu, DH [1 ]
Zhu, HY [1 ]
Zhu, QR [1 ]
机构
[1] Jilin Univ, Inst Atom & Mol Phys, Changchun 130012, Peoples R China
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中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present a scheme aiming at the field-free orientation of molecules with smaller permanent dipole moments under the framework of the half-cycle pulse (HCP) method. Taking the HCCCI molecule as an example, we show that a. train of identical HCPs with special time intervals can considerably raise the level of the orientation. The scheme is analytically interpreted in terms of intermittent Rabi oscillations by referring to a simplified two-state model.
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页码:576 / 579
页数:4
相关论文
共 15 条
[1]   Phase modulation of ultrashort light pulses using molecular rotational wave packets [J].
Bartels, RA ;
Weinacht, TC ;
Wagner, N ;
Baertschy, M ;
Greene, CH ;
Murnane, MM ;
Kapteyn, HC .
PHYSICAL REVIEW LETTERS, 2002, 88 (01) :4-139034
[2]  
Brooks P.R., 1976, SCIENCE, V11, P193
[3]   Time-dependent alignment and orientation of molecules in combined electrostatic and pulsed nonresonant laser fields [J].
Cai, L ;
Marango, J ;
Friedrich, B .
PHYSICAL REVIEW LETTERS, 2001, 86 (05) :775-778
[4]  
COHENTANNOUDJI C, 1977, QUANTUM MECHANICS, P413
[5]   Two-frequency IR laser orientation of polar molecules. Numerical simulations for HCN [J].
Dion, CM ;
Bandrauk, AD ;
Atabek, O ;
Keller, A ;
Umeda, H ;
Fujimura, Y .
CHEMICAL PHYSICS LETTERS, 1999, 302 (3-4) :215-223
[6]   Numerical simulation of the isomerization of HCN by two perpendicular intense IR laser pulses [J].
Dion, CM ;
Chelkowski, S ;
Bandrauk, AD ;
Umeda, H ;
Fujimura, Y .
JOURNAL OF CHEMICAL PHYSICS, 1996, 105 (20) :9083-9092
[7]   Manipulating molecules via combined static and laser fields [J].
Friedrich, B ;
Herschbach, D .
JOURNAL OF PHYSICAL CHEMISTRY A, 1999, 103 (49) :10280-10288
[8]  
Haj-Yedder A.Ben., 2002, Physical Review A, V66, P063401
[9]   Generation of single dispersion precompensated 1-fs pulses by shaped-pulse optimized high-order stimulated Raman scattering [J].
Kalosha, V ;
Spanner, M ;
Herrmann, J ;
Ivanov, M .
PHYSICAL REVIEW LETTERS, 2002, 88 (10) :4-103901
[10]   Electromagnetic bubble generation by half-cycle pulses [J].
Kaplan, AE ;
Straub, SF ;
Shkolnikov, PL .
OPTICS LETTERS, 1997, 22 (06) :405-407