Origin of the boson peak in a network glass B2O3

被引:49
作者
Engberg, D
Wischnewski, A
Buchenau, U
Börjesson, L
Dianoux, AJ
Sokolov, AP
Torell, LM
机构
[1] Chalmers, Dept Expt Phys, S-41296 Gothenburg, Sweden
[2] Forschungszentrum Julich, Inst Festkorperforsch, D-52425 Julich, Germany
[3] Chalmers, Dept Appl Phys, S-41296 Gothenburg, Sweden
[4] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France
关键词
D O I
10.1103/PhysRevB.59.4053
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report coherent inelastic neutron-scattering spectra for the network glass former B2O3, measured at temperatures from 100 to 1300 K (T-g similar to 525 K). At the first sharp diffraction peak, which stems from the van der Waals packing of layerlike units, one finds a correlated in-phase motion of these units at low frequency, and in addition a quasi-incoherent contribution for all temperatures. The contribution of the in-phase motion in the frequency range of the boson peak and the fast relaxations is significantly higher than the one expected for the sound waves.
引用
收藏
页码:4053 / 4057
页数:5
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  • [1] Evidence of high frequency propagating modes in vitreous silica
    Benassi, P
    Krisch, M
    Masciovecchio, C
    Mazzacurati, V
    Monaco, G
    Ruocco, G
    Sette, F
    Verbeni, R
    [J]. PHYSICAL REVIEW LETTERS, 1996, 77 (18) : 3835 - 3838
  • [2] IS THERE A CORRELATION BETWEEN THE 1ST SHARP DIFFRACTION PEAK AND THE LOW-FREQUENCY VIBRATIONAL BEHAVIOR OF GLASSES
    BORJESSON, L
    HASSAN, AK
    SWENSON, J
    TORELL, LM
    FONTANA, A
    [J]. PHYSICAL REVIEW LETTERS, 1993, 70 (09) : 1275 - 1278
  • [3] LOW-ENERGY MODES IN PHOSPHATE-GLASSES - A COMPARISON WITH THE SOFT POTENTIAL MODEL
    BRODIN, A
    FONTANA, A
    BORJESSON, L
    CARINI, G
    TORELL, LM
    [J]. PHYSICAL REVIEW LETTERS, 1994, 73 (15) : 2067 - 2070
  • [4] Is the fast process at the glass transition mainly due to long wavelength excitations?
    Buchenau, U
    Wischnewski, A
    Richter, D
    Frick, B
    [J]. PHYSICAL REVIEW LETTERS, 1996, 77 (19) : 4035 - 4038
  • [5] LOW-FREQUENCY MODES IN VITREOUS SILICA
    BUCHENAU, U
    PRAGER, M
    NUCKER, N
    DIANOUX, AJ
    AHMAD, N
    PHILLIPS, WA
    [J]. PHYSICAL REVIEW B, 1986, 34 (08): : 5665 - 5673
  • [6] Neutron scattering evidence for localized soft modes in amorphous polymers
    Buchenau, U
    Pecharroman, C
    Zorn, R
    Frick, B
    [J]. PHYSICAL REVIEW LETTERS, 1996, 77 (04) : 659 - 662
  • [7] INELASTIC NEUTRON-SCATTERING FROM AMORPHOUS SOLIDS .1. CALCULATION OF SCATTERING LAW FOR MODEL STRUCTURES
    CARPENTER, JM
    PELIZZARI, CA
    [J]. PHYSICAL REVIEW B, 1975, 12 (06): : 2391 - 2396
  • [8] High frequency sounds waves in vitreous silica
    Dell'Anna, R
    Ruocco, G
    Sampoli, M
    Viliani, G
    [J]. PHYSICAL REVIEW LETTERS, 1998, 80 (06) : 1236 - 1239
  • [9] Floppy modes in crystalline and amorphous silicates
    Dove, MT
    Harris, MJ
    Hannon, AC
    Parker, JM
    Swainson, IP
    Gambhir, M
    [J]. PHYSICAL REVIEW LETTERS, 1997, 78 (06) : 1070 - 1073
  • [10] Sound waves and other modes in the strong glass former B2O3
    Engberg, D
    Wischnewski, A
    Buchenau, U
    Borjesson, L
    Dianoux, AJ
    Sokolov, AP
    Torell, LM
    [J]. PHYSICAL REVIEW B, 1998, 58 (14) : 9087 - 9097