Fabrication of bismuth oxide/titanium dioxide nano-tube arrays photoelectrode and its enhanced visible light photocatalytic performance for degradation of 4-chlorphenol

被引：13

作者：

Cui, Yuqi ^{[1
,2
]}

Zhang, Huixuan ^{[1
,2
]}

Guo, Ruonan ^{[1
,2
]}

Ma, Qiuling ^{[1
,2
]}

Deng, Xiaoyong ^{[1
,2
]}

Cheng, Xiuwen ^{[1
,2
,4
,5
]}

Li, Xiaoli ^{[1
,2
]}

Xie, Mingzheng ^{[1
,2
]}

Cheng, Qingfeng ^{[3
]}

Zou, Changwu ^{[3
]}

机构：

[1] Lanzhou Univ, Coll Earth & Environm Sci, Minist Educ, Key Lab Western Chinas Environm Syst, Lanzhou 730000, Gansu, Peoples R China

[2] Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China

[3] Chengdu Univ Informat Technol, Coll Resources & Environm, Chengdu 610225, Sichuan, Peoples R China

[4] Nanjing Univ Informat Sci & Technol, Collaborat Innovat Ctr Atmospher Environm & Equip, Sch Environm Sci & Engn, Jiangsu Engn Technol Res Ctr Environm Cleaning Ma, Nanjing 210044, Jiangsu, Peoples R China

[5] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 2000050, Peoples R China

来源：

ELECTROCHIMICA ACTA | 2017年 / 246卷

基金：

中国国家自然科学基金;

关键词：

Bi2O3/TiO2 nano-tube arrays; Photoelectrode; Visible light; Photocatalysis; 4-chlorphenol; TIO2 NANOTUBES PHOTOELECTRODE; HYDROTHERMAL SYNTHESIS; CONSTRUCTION; IRRADIATION; REDUCTION; COMPOSITE; FACILE; HETEROJUNCTION; DICLOFENAC; EFFICIENCY;

D O I：

10.1016/j.electacta.2017.06.153

中图分类号：

O646 [电化学、电解、磁化学];

学科分类号：

081704 ;

摘要：

In order to improve the photocatalytic (PC) performance of TiO2 nano-material, TiO2 nanotube arrays (NTAs) was fabricated by anodization. Subsequently, Bi2O3 nano-particles were successfully deposited onto the surface of TiO2 NTAs through galvanostatic electrodeposition strategy. Afterwards, series of characterizations including scanning electron microscope (SEM), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), Ultraviolet-visible diffuse reflectance spectroscopy (UV-vis DRS) and photoelectrochemical (PECH) measurements were applied to clarify physicochemical properties of the as-fabricated Bi2O3/TiO2 NTAs photoelectrode. All results indicated that the light absorbance and photoinduced charge separation efficiency of Bi2O3/TiO2 NTAs photoelectrode were significantly improved. As expected, Bi2O3/TiO2 NTAs photoelectrode displayed higher PC efficiency for degradation of 4-chlorphenol (4-CP) aqueous solution than that of pristine TiO2 NTAs. Besides these, the enhanced visible light PC mechanism was proposed. Furthermore, Bi2O3/TiO2 NTAs photoelectrode performed good reusability and stability even after six recycle utilization. (C) 2017 Elsevier Ltd. All rights reserved.

引用

页码：1075 / 1081

页数：7

共 31 条

[1] In situ ion exchange synthesis of the novel Ag/AgBr/BiOBr hybrid with highly efficient decontamination of pollutants [J].

Cheng, Hefeng ;

Huang, Baibiao ;

Wang, Peng ;

Wang, Zeyan ;

Lou, Zaizhu ;

Wang, Junpeng ;

Qin, Xiaoyan ;

Zhang, Xiaoyang ;

Dai, Ying .

CHEMICAL COMMUNICATIONS, 2011, 47 (25) :7054-7056

[2] A facile and novel strategy to synthesize reduced TiO2 nanotubes photoelectrode for photoelectrocatalytic degradation of diclofenac [J].

Cheng, Xiuwen ;

Cheng, Qingfeng ;

Deng, Xiaoyong ;

Wang, Pu ;

Liu, Huiling .

CHEMOSPHERE, 2016, 144 :888-894

[3] Construction of TiO2 nano-tubes arrays coupled with Ag2S nano-crystallites photoelectrode and its enhanced visible light photocatalytic performance and mechanism [J].

Cheng, Xiuwen ;

Cheng, Qingfeng ;

Deng, Xiaoyong ;

Wang, Pu ;

Liu, Huiling .

ELECTROCHIMICA ACTA, 2015, 184 :264-275

[4] One-step construction of N/Ti3+ codoped TiO2 nanotubes photoelectrode with high photoelectrochemical and photoelectrocatalytic performance [J].

Cheng, Xiuwen ;

Cheng, Qingfeng ;

Li, Bo ;

Deng, Xiaoyong ;

Li, Junjing ;

Wang, Pu ;

Zhang, Baoqing ;

Liu, Huiling ;

Wang, Xiaoning .

ELECTROCHIMICA ACTA, 2015, 186 :442-448

[5] Preparation of graphene film decorated TiO2 nano-tube array photoelectrode and its enhanced visible light photocatalytic mechanism [J].

Cheng, Xiuwen ;

Liu, Huiling ;

Chen, Qinghua ;

Li, Junjing ;

Wang, Pu .

CARBON, 2014, 66 :450-458

[6] Preparation and characterization of palladium nano-crystallite decorated TiO2 nano-tubes photoelectrode and its enhanced photocatalytic efficiency for degradation of diclofenac [J].

Cheng, Xiuwen ;

Liu, Huiling ;

Chen, Qinghua ;

Li, Junjing ;

Wang, Pu .

JOURNAL OF HAZARDOUS MATERIALS, 2013, 254 :141-148

[7] Low temperature one-step synthesis of rutile TiO2/BiOCl composites with enhanced photocatalytic activity [J].

Duo, Fangfang ;

Wang, Yawen ;

Fan, Caimei ;

Mao, Xiaoming ;

Zhang, Xiaochao ;

Wang, Yunfang ;

Liu, Jianxin .

MATERIALS CHARACTERIZATION, 2015, 99 :8-16

[8]

Hezama K. Abdo, 2017, CERAM INT, V43, P5292

[9] Ordered macroporous Bi2O3/TiO2 film coated on a rotating disk with enhanced photocatalytic activity Under visible irradiation [J].

Huo, Yuning ;

Chen, Xiaofang ;

Zhang, Jia ;

Pan, Gaifang ;

Jia, Jinping ;

Li, Hexing .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2014, 148 :550-556

[10] Detection of active oxidative species in TiO2 photocatalysis using the fluorescence technique [J].

Ishibashi, K ;

Fujishima, A ;

Watanabe, T ;

Hashimoto, K .

ELECTROCHEMISTRY COMMUNICATIONS, 2000, 2 (03) :207-210

← 1 2 3 4 →