Low-Cost Route for Preparing Carbon-Silica Composite Mesoporous Material from Coal Gasification Slag: Synthesis, Characterization and Application in Purifying Dye Wastewater

被引:28
作者
Liu, Shuo [1 ]
Wei, Jilun [2 ]
Chen, Xingtong [1 ]
Ai, Weidong [1 ]
Wei, Cundi [1 ]
机构
[1] Jilin Univ, Coll Mat Sci & Engn, Key Lab Automobile Mat, Minist Educ, Changchun 130025, Jilin, Peoples R China
[2] Arizona State Univ, Dept Chem, Coll Liberal Art & Sci, Tempe, AZ 85381 USA
关键词
Coal slag; Low-cost preparation; Mesoporous carbon; Mesoporous silica; Dye adsorption; RESIDUAL CARBON; SURFACE-AREA; ADSORPTION; REMOVAL; BIOMASS; ACID;
D O I
10.1007/s13369-020-04383-z
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The promotion of China's coal gasification industry has produced highly yielded coal gasification slag. This research utilized the coal gasification fine slag as raw material and successfully synthesized a carbon-silica composite mesoporous material with a specific surface area of 500 m(2)/g and pore volume of 0.54 cm(3)/g by simple acid leaching technology. The influence of reaction conditions on porosity was discussed in detail, and the optimal sample was characterized by N-2 adsorption/desorption analyzer, SEM, TEM and others. Also, by the methylene blue adsorption experiment, we confirmed that the maximum adsorption capacity of synthesized mesoporous material is 182.48 mg/g, showing that it can be envisioned as a competitive candidate for purification of textile industrial wastewater.
引用
收藏
页码:4647 / 4657
页数:11
相关论文
共 28 条
[1]   Recent advances in new generation dye removal technologies: novel search for approaches to reprocess wastewater [J].
Ahmad, Akil ;
Mohd-Setapar, Siti Hamidah ;
Chuong, Chuo Sing ;
Khatoon, Asma ;
Wani, Waseem A. ;
Kumar, Rajeev ;
Rafatullah, Mohd .
RSC ADVANCES, 2015, 5 (39) :30801-30818
[2]   Mesoporous carbon nanomaterials induced pulmonary surfactant inhibition, cytotoxicity, inflammation and lung fibrosis [J].
Chen, Yunan ;
Yang, Yi ;
Xu, Bolong ;
Wang, Shunhao ;
Li, Bin ;
Ma, Juan ;
Gao, Jie ;
Zuo, Yi Y. ;
Liu, Sijin .
JOURNAL OF ENVIRONMENTAL SCIENCES, 2017, 62 :100-114
[3]   Development of CO2 activated biochar from solid wastes of a beer industry and its application for methylene blue adsorption [J].
Franciski, Mauro A. ;
Peres, Enrique C. ;
Godinho, Marcelo ;
Perondi, Daniele ;
Foletto, Edson L. ;
Collazzo, Gabriela C. ;
Dotto, Guilherme L. .
WASTE MANAGEMENT, 2018, 78 :630-638
[4]   A carbon silica composite prepared from water slurry coal gasification slag [J].
Gu, Yu-yan ;
Qiao, Xiu-chen .
MICROPOROUS AND MESOPOROUS MATERIALS, 2019, 276 :303-307
[5]  
Heibati B, 2014, J IND ENG CHEM, V20, P2939
[6]   Synthesis of pore-expanded mesoporous materials using waste quartz sand and the adsorption effects of methylene blue [J].
Hong, Jun-Ming ;
Lin, Bing ;
Jiang, Jie-Shan ;
Chen, Bor-Yann ;
Chang, Chang-Tang .
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY, 2014, 20 (05) :3667-3671
[7]   Mesoporous activated carbon prepared from NaOH activation of rattan (Lacosperma secundiflorum) hydrochar for methylene blue removal [J].
Islam, Md. Azharul ;
Ahmed, M. J. ;
Khanday, W. A. ;
Asif, M. ;
Hameed, B. H. .
ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY, 2017, 138 :279-285
[8]   A new approach to prepare mesoporous silica using coal fly ash [J].
Li, Chen-chen ;
Qiao, Xiu-chen .
CHEMICAL ENGINEERING JOURNAL, 2016, 302 :388-394
[9]   Large surface area MCM-41 prepared from acid leaching residue of coal gasification slag [J].
Li, Chen-chen ;
Qiao, Xiu-chen ;
Yu, Jian-guo .
MATERIALS LETTERS, 2016, 167 :246-249
[10]   A new method to prepare mesoporous silica from coal gasification fine slag and its application in methylene blue adsorption [J].
Liu, Shuo ;
Chen, Xingtong ;
Ai, Weidong ;
Wei, Cundi .
JOURNAL OF CLEANER PRODUCTION, 2019, 212 :1062-1071