Time-resolved collapse and revival of the Kondo state near a quantum phase transition

被引:18
|
作者
Wetli, C. [1 ]
Pal, S. [1 ]
Kroha, J. [2 ,3 ,4 ]
Kliemt, K. [5 ]
Krellner, C. [5 ]
Stockert, O. [6 ]
von Loehneysen, H. [7 ,8 ]
Fiebig, M. [1 ]
机构
[1] Swiss Fed Inst Technol, Dept Mat, Zurich, Switzerland
[2] Univ Bonn, Inst Phys, Bonn, Germany
[3] Univ Bonn, Bethe Ctr Theoret Phys, Bonn, Germany
[4] Zhejiang Univ, Ctr Correlated Matter, Hangzhou, Zhejiang, Peoples R China
[5] Goethe Univ Frankfurt, Inst Phys, Frankfurt, Germany
[6] Max Planck Inst Chem Phys Solids, Dresden, Germany
[7] Karlsruhe Inst Technol, Inst Festkorperphys, Karlsruhe, Germany
[8] Karlsruhe Inst Technol, Inst Phys, Karlsruhe, Germany
关键词
FERMI-LIQUID BEHAVIOR; HEAVY; ANTIFERROMAGNETISM; TEMPERATURE; DYNAMICS; SYSTEMS;
D O I
10.1038/s41567-018-0228-3
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
One of the most successful paradigms of many-body physics is the concept of quasiparticles: excitations in strongly interacting matter behaving like weakly interacting particles in free space. Quasiparticles in metals are very robust objects. Nevertheless, when a system's ground state undergoes a qualitative change at a quantum critical point (QCP)(1), the quasiparticles may disintegrate and give way to an exotic quantum-fluid state of matter. The nature of this breakdown is intensely debated(2-5), because the emergent quantum fluid dominates material properties up to high temperatures and might even be related to the occurrence of superconductivity in some compounds(6). Here we trace the dynamics of heavy-fermion quasiparticles in CeCu6-xAux and monitor their evolution towards the QCP in time-resolved experiments, supported by many-body calculations. A terahertz pulse disrupts the many-body heavy-fermion state. Under emission of a delayed, phase-coherent terahertz reflex the heavy-fermion state recovers, with a coherence time 100 times longer than typically associated with correlated metals(7,8). The quasiparticle weight collapses towards the QCP, yet its formation temperature remains constant-phenomena believed to be mutually exclusive. Coexistence in the same experiment calls for revisions in our view on quantum criticality.
引用
收藏
页码:1103 / +
页数:6
相关论文
共 50 条
  • [41] Magnetic quantum phase transition in an anisotropic kondo lattice
    Glossop, Matthew T.
    Ingersent, Kevin
    PHYSICAL REVIEW LETTERS, 2007, 99 (22)
  • [42] Solid-state transition mechanism in carbamazepine polymorphs by time-resolved terahertz spectroscopy
    Zeitler, J. Axel
    Taday, Philip F.
    Gordon, Keith C.
    Pepper, Michael
    Rades, Thomas
    CHEMPHYSCHEM, 2007, 8 (13) : 1924 - 1927
  • [43] TIME-RESOLVED AND PHASE-RESOLVED ROTATIONAL DIFFUSION MEASUREMENTS
    WIRTH, MJ
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1987, 194 : 101 - ANYL
  • [44] A steady-state and time-resolved photophysical study of CdTe quantum dots in water
    Iagatti, Alessandro
    Tarpani, Luigi
    Fiacchi, Eleonora
    Bussotti, Laura
    Marcelli, Agnese
    Foggi, Paolo
    Latterini, Loredana
    PHOTOCHEMICAL & PHOTOBIOLOGICAL SCIENCES, 2015, 14 (02) : 397 - 406
  • [45] Time-resolved and steady-state FRET spectroscopy on commercial biocompatible quantum dots
    Wegner, D.
    Geissler, D.
    Stufler, S.
    Loehmannsroeben, H. -G.
    Hildebrandt, N.
    COLLOIDAL QUANTUM DOTS/NANOCRYSTALS FOR BIOMEDICAL APPLICATIONS VI, 2011, 7909
  • [46] A steady-state and time-resolved photophysical study of CdTe quantum dots in water
    Alessandro Iagatti
    Luigi Tarpani
    Eleonora Fiacchi
    Laura Bussotti
    Agnese Marcelli
    Paolo Foggi
    Loredana Latterini
    Photochemical & Photobiological Sciences, 2015, 14 : 397 - 406
  • [47] Time-resolved measurements of an ion channel conformational change driven by a membrane phase transition
    Stevenson, Paul
    Tokmakoff, Andrei
    PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2017, 114 (41) : 10840 - 10845
  • [48] TIME-RESOLVED OBSERVATION OF PHOTOCHEMICAL PHASE-TRANSITION IN POLYMER LIQUID-CRYSTALS
    SASAKI, T
    IKEDA, T
    ICHIMURA, K
    MACROMOLECULES, 1992, 25 (14) : 3807 - 3811
  • [49] Time-resolved structural study of the Ge(111) high-temperature phase transition
    Dept. of Elec. and Comp. Engineering, Old Dominion University, Norfolk, VA 23529, United States
    Surf Sci, 1-3 (95-102):
  • [50] Time-resolved photoluminescence near Fermi level in a field-induced quantum dot lattice
    Hammura, K
    Nomura, S
    Aoyagi, Y
    PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 2002, 13 (2-4): : 251 - 254