Effects of surface oxide films on hydrogen permeation and susceptibility to embrittlement of X80 steel under hydrogen atmosphere

被引：54

作者：

Zhang, Timing ^{[1
]}

Zhao, Weimin ^{[1
]}

Zhao, Yujiao ^{[1
]}

Ouyang, Kai ^{[1
]}

Deng, Qiushi ^{[1
]}

Wang, Yonglin ^{[1
]}

Jiang, Wei ^{[1
]}

机构：

[1] China Univ Petr, Coll Mech & Elect Engn, Qingdao 266580, Peoples R China

来源：

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2018年 / 43卷 / 06期

基金：

中国国家自然科学基金; 中国博士后科学基金;

关键词：

Oxide films; X80; steel; Hydrogen permeation; SSRT; Hydrogen embrittlement; COAL-GAS ENVIRONMENT; PIPELINE STEEL; FRACTURE-TOUGHNESS; STRESS-CORROSION; STAINLESS-STEEL; WELDED-JOINTS; ENERGY; TITANIUM; SYSTEMS; CRACKING;

D O I：

10.1016/j.ijhydene.2017.12.170

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Hydrogen embrittlement (HE) induced by hydrogen permeation is a serious threat to the hydrogen transmission pipeline. In this study, oxide films were prepared on X80 steel by applying high-temperature oxidation, blackening treatment and passivation in concentrated H2SO4, and their effects on hydrogen permeation and HE susceptibility of X80 substrate were studied by conducting hydrogen permeation tests and slow strain rate tension (SSRT) tests. A numerical diffusion model was established to quantitatively determine the resistance of these oxide films to hydrogen permeation. Results showed that the oxide film prepared by high-temperature oxidation presented the highest resistance to hydrogen permeation with the phi(m)/phi(f) value of 3828, and the corresponding HE index decreased from 38.07% for bare X80 steel to only 4.00% for that covered with oxide film. The characteristic of the corresponding fracture surfaces changed from brittle features such as quasi cleavage facets and secondary cracks to typical ductile dimple feature. (C) 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

引用

页码：3353 / 3365

页数：13

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