Self-assembly of an organic-inorganic hybrid nanoflower as an efficient biomimetic catalyst for self-activated tandem reactions

被引:159
作者
Huang, Yanyan [1 ,2 ]
Ran, Xiang [1 ,2 ]
Lin, Youhui [1 ,2 ]
Ren, Jinsong [1 ]
Qu, Xiaogang [1 ]
机构
[1] Chinese Acad Sci, Changchun Inst Appl Chem, Grad Sch, Biol Chem Lab, Changchun 130022, Jilin, Peoples R China
[2] Chinese Acad Sci, Changchun Inst Appl Chem, Grad Sch, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Jilin, Peoples R China
基金
中国国家自然科学基金;
关键词
CERIUM OXIDE NANOPARTICLES; PEROXIDASE-LIKE ACTIVITY; GOLD NANOPARTICLES; ARTIFICIAL ENZYMES; HYDROGEN-PEROXIDE; MIMIC PEROXIDASE; FACILE SYNTHESIS; GLUCOSE; NANOCOMPOSITES; NANOMATERIALS;
D O I
10.1039/c5cc00040h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The BSA-Cu-3(PO4)(2)center dot 3H(2)O hybrid nanoflower was used as a biomimetic catalyst with excellent catalytic activity, durability and stability. When GOx was used as the protein component, this composite could realize self-activated cascade catalysis. Our nanoflower system could also be used to decompose organic pollutants with high efficiency.
引用
收藏
页码:4386 / 4389
页数:4
相关论文
共 34 条
[1]   Oxidase-Like Activity of Polymer-Coated Cerium Oxide Nanoparticles [J].
Asati, Atul ;
Santra, Santimukul ;
Kaittanis, Charalambos ;
Nath, Sudip ;
Perez, J. Manuel .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2009, 48 (13) :2308-2312
[2]   Photosynthetic energy conversion: natural and artificial [J].
Barber, James .
CHEMICAL SOCIETY REVIEWS, 2009, 38 (01) :185-196
[3]   Biomimetic reactions catalyzed by cyclodextrins and their derivatives [J].
Breslow, R ;
Dong, SD .
CHEMICAL REVIEWS, 1998, 98 (05) :1997-2011
[4]   Helical Carbon Nanotubes: Intrinsic Peroxidase Catalytic Activity and Its Application for Biocatalysis and Biosensing [J].
Cui, Rongjing ;
Han, Zhida ;
Zhu, Jun-Jie .
CHEMISTRY-A EUROPEAN JOURNAL, 2011, 17 (34) :9377-9384
[5]   Graphene oxide-Fe3O4 magnetic nanocomposites with peroxidase-like activity for colorimetric detection of glucose [J].
Dong, Ya-lei ;
Zhang, Hui-ge ;
Rahman, Zia Ur ;
Su, Li ;
Chen, Xiao-jiao ;
Hu, Jing ;
Chen, Xing-guo .
NANOSCALE, 2012, 4 (13) :3969-3976
[6]   CuS nanoparticles as a mimic peroxidase for colorimetric estimation of human blood glucose level [J].
Dutta, Amit Kumar ;
Das, Sudipto ;
Samanta, Suvendu ;
Samanta, Partha Kumar ;
Adhikary, Bibhutosh ;
Biswas, Papu .
TALANTA, 2013, 107 :361-367
[7]   Interenzyme Substrate Diffusion for an Enzyme Cascade Organized on Spatially Addressable DNA Nanostructures [J].
Fu, Jinglin ;
Liu, Minghui ;
Liu, Yan ;
Woodbury, Neal W. ;
Yan, Hao .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (12) :5516-5519
[8]   Intrinsic peroxidase-like activity of ferromagnetic nanoparticles [J].
Gao, Lizeng ;
Zhuang, Jie ;
Nie, Leng ;
Zhang, Jinbin ;
Zhang, Yu ;
Gu, Ning ;
Wang, Taihong ;
Feng, Jing ;
Yang, Dongling ;
Perrett, Sarah ;
Yan, Xiyun .
NATURE NANOTECHNOLOGY, 2007, 2 (09) :577-583
[9]  
Ge J, 2012, NAT NANOTECHNOL, V7, P428, DOI [10.1038/nnano.2012.80, 10.1038/NNANO.2012.80]
[10]   Towards Chemical Communication between Gated Nanoparticles [J].
Gimenez, Cristina ;
Climent, Estela ;
Aznar, Elena ;
Martinez-Manez, Ramon ;
Sancenon, Felix ;
Dolores Marcos, M. ;
Amoros, Pedro ;
Rurack, Knut .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2014, 53 (46) :12629-12633